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P. Maksyutenko, P. P. Radi, D. N. Kozlov and A. P. Kouzov Polarization- and time-resolved DFWM spectroscopy of the A 2Σ+− X 2Π (0,0) band transitions of nascent OH radicals generated by 266 nm laser photolysis of H2O2 Journal of Raman Spectroscopy 44

Version of Record online: 15 MAY 2013 | DOI: 10.1002/jrs.4299

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Degenerate four-wave mixing is used to measure the line shapes of specific rovibrational transitions in the A2Σ+ - X2Π (0,0) band of nascent OH radicals upon pulsed photo-dissociation of H2O2. Isotropic and anisotropic components of the non-linear susceptibility tensor are separately accessible by using appropriate polarization geometries. In particular, four-wave mixing signals can be generated that are exclusively due to the occurrence of the transient anisotropy of the recoil velocity and angular momentum vector distributions of the fragments emerging from the dissociation reaction.

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