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Jing Yang Quek, Peter J. Roth, Richard A. Evans, Thomas P. Davis and Andrew B. Lowe Reversible addition–fragmentation chain transfer synthesis of amidine-based, CO2-responsive homo and AB diblock (Co)polymers comprised of histamine and their gas-triggered self-assembly in water Journal of Polymer Science Part A: Polymer Chemistry 51

Version of Record online: 29 OCT 2012 | DOI: 10.1002/pola.26397

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Gas responsive homo- and AB diblock copolymers based on histamine and arginine have been prepared via RAFT polymerization employing activated ester chemistry. Quantitative formation of histamine and arginine (co)polymers was verified by 1H NMR spectroscopy giving stimulus responsive materials capable of undergoing reversible self-assembly employing CO2/H2O and N2 as triggers.

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