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Ulrich Mansfeld, Andreas Winter, Martin D. Hager, Wolfgang Günther, Esra Altuntaş and Ulrich S. Schubert A Homotelechelic bis-terpyridine macroligand: One-step synthesis and its metallo-supramolecular self-assembly Journal of Polymer Science Part A: Polymer Chemistry 51

Version of Record online: 14 FEB 2013 | DOI: 10.1002/pola.26586

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A homodifunctional initiator was designed and applied for the controlled nitroxide-mediated polymerization of styrene to yield a α,ω-homotelechelic macroligand featuring two terpyridine moieties as designated metal binding sites. The self-assembly with FeII ions into a chain-extended metallopolymer and the disassembly thereof in the presence of a strong competitive ligand was investigated by UV–vis absorption spectroscopy and diffusion-ordered NMR spectroscopy.

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