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Markus Ernst Gruner Trends in spin and orbital magnetism of free and encapsulated FePt nanoparticles physica status solidi (a) 210

Article first published online: 4 JUN 2013 | DOI: 10.1002/pssa.201329048

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Large-scale first principles calculations in the framework of density functional theory offer detailed insight into the close interrelation between particle composition, morphology and magnetism with electronic resolution. Exploiting the power of contemporary supercomputers, one can identify systematic trends in spin and orbital magnetism of nanometer-sized hard magnetic particles related to their structure or chemical environment. This Feature Article concentrates on Fe-Pt nanoparticles, which are considered as promising candidates for ultra-high density recording media. Special emphasis is made on the role of the surfaces and the impact of a protective encapsulation with Cu, Au, Al or further main group elements on the hard magnetic properties. The anisotropy of the orbital moments turns out to be a valuable quantity characterizing the particular contribution of surfaces and interfaces on the atomic scale.

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