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Lei Liao, Zehao Song, Yu Zhou, Huan Wang, Qin Xie, Hailin Peng and Zhongfan Liu Photoinduced Methylation of Graphene Small 9

Article first published online: 20 MAR 2013 | DOI: 10.1002/smll.201203069

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Covalent grafting of methyl groups onto the basal plane of graphene is achieved through a photochemical reaction between graphene and di-tert-butyl peroxide. The methylation of graphene is found to be reversible. The edge of single-layer graphene shows the largest methylation reactivity, which provides a route to tailor the edge state of graphene.

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