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  1. From Flatland to Spaceland: Higher Dimensional Patterning with Two-Dimensional Materials

    Po-Yen Chen, Muchun Liu, Zhongying Wang, Robert H. Hurt and Ian Y. Wong

    Version of Record online: 28 FEB 2017 | DOI: 10.1002/adma.201605096

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    Emerging approaches to fabrication of 3D architectures are discussed, emphasizing creation of textural patterns by directed assembly of nanosheet building blocks: (1) wrinkling and crumpling of 2D material films; (2) wrapping and crumpling of 2D materials around curved objects; (3) folding (origami) and cutting (kirigami) using 2D materials; and (4) 3D printing from 2D nanosheet suspensions.

  2. Advances in Subcritical Hydro-/Solvothermal Processing of Graphene Materials

    Suchithra Padmajan Sasikala, Philippe Poulin and Cyril Aymonier

    Version of Record online: 28 FEB 2017 | DOI: 10.1002/adma.201605473

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    The subcritical hydro-/solvothermal synthesis method is a very promising green alternative to many conventional synthesis methods of graphene and its associated materials. This review elaborates on important developments in subcritical hydro-/solvothermal syntheses of graphene based functional materials and classifies their application.

  3. Asymmetric Supercapacitor Electrodes and Devices

    Nitin Choudhary, Chao Li, Julian Moore, Narasimha Nagaiah, Lei Zhai, Yeonwoong Jung and Jayan Thomas

    Version of Record online: 28 FEB 2017 | DOI: 10.1002/adma.201605336

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    Recent developments in asymmetric supercapacitor (ASC) electrode materials (anode and cathode) including carbonaceous materials, metal oxides/nitrides, conductive polymers, and 2D materials are highlighted. A rational electrode material design with tailored nanostructures endows significant improvement in the specific capacitance and energy density of ASCs. The resulting ASCs have the potential to function as a fast charging energy source for next-generation flexible electronics, e-textiles, and transportation applications.

  4. Coordination Polymers Derived General Synthesis of Multishelled Mixed Metal-Oxide Particles for Hybrid Supercapacitors

    Bu Yuan Guan, Akihiro Kushima, Le Yu, Sa Li, Ju Li and Xiong Wen (David) Lou

    Version of Record online: 28 FEB 2017 | DOI: 10.1002/adma.201605902

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    A general method is developed to synthesize highly complex multishelled mixed metal-oxide particles with tunable size and composition from the pyrolysis of a novel class of amorphous coordination polymers. With the structural and compositional advantages, the unique seven-shelled NiCo2O4 particles exhibit remarkable electrochemical performance as an electrode material for hybrid supercapacitors.

  5. Naphthobischalcogenadiazole Conjugated Polymers: Emerging Materials for Organic Electronics

    Itaru Osaka and Kazuo Takimiya

    Version of Record online: 27 FEB 2017 | DOI: 10.1002/adma.201605218

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    π-Conjugated polymers are an important class of materials for organic electronics. This article focuses on the recent advances of emerging π-conjugated polymers incorporating naphthobischalcogenadiazoles such as naphthobisoxadiazole, naphthobisthiadiazole, and naphthobisselenadiazle as strong acceptor building unit. The molecular design, synthesis, electronic properties, ordering structures, and device applications of these polymers are also discussed.

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