Advanced Synthesis & Catalysis

Cover image for Vol. 358 Issue 3

Early View (Online Version of Record published before inclusion in an issue)

Editor: Joe P. Richmond, Chairman of the Editorial Board: Eric N. Jacobsen

Impact Factor: 5.663

ISI Journal Citation Reports © Ranking: 2014: 2/72 (Chemistry Applied); 6/58 (Chemistry Organic)

Online ISSN: 1615-4169

Associated Title(s): Angewandte Chemie International Edition, Asian Journal of Organic Chemistry, Chemistry - A European Journal, Chemistry – An Asian Journal, ChemCatChem, European Journal of Organic Chemistry

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  1. Communications

  2. Updates

  3. Full Papers

    1. Very Important Publication

      Easy Access to 1-Amino and 1-Carbon Substituted Isoquinolines via Cobalt-Catalyzed C[BOND]H/N[BOND]O Bond Activation

      Krishnamoorthy Muralirajan, Ramajayam Kuppusamy, Sekar Prakash and Chien-Hong Cheng

      Article first published online: 11 FEB 2016 | DOI: 10.1002/adsc.201501056

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    2. Titania-Supported Gold Nanoparticles Catalyze the Selective Oxidation of Amines into Nitroso Compounds in the Presence of Hydrogen Peroxide

      Stella Fountoulaki, Petros L. Gkizis, Theodoros S. Symeonidis, Eleni Kaminioti, Athanasia Karina, Ioannis Tamiolakis, Gerasimos S. Armatas and Ioannis N. Lykakis

      Article first published online: 11 FEB 2016 | DOI: 10.1002/adsc.201500957

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  4. Communications

    1. Efficient Oxidative Cleavage of Tetrahydrofuran-2-methanols to γ-Lactones by a 2-Iodobenzamide Catalyst in Combination with Oxone®

      Takayuki Yakura, Yuto Horiuchi, Yushi Nishimura, Akihiro Yamada, Hisanori Nambu and Tomoya Fujiwara

      Article first published online: 11 FEB 2016 | DOI: 10.1002/adsc.201500795

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    2. Organophotocatalytic Synthesis of Phosphoramidates

      Marta Meazza, Agnieszka Kowalczuk, Luke Shirley, Jung Woon Yang, Hao Guo and Ramon Rios

      Article first published online: 11 FEB 2016 | DOI: 10.1002/adsc.201501068

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    3. Very Important Publication

      Iridium-Catalyzed Transfer Hydrogenation of 1,10-Phenanthrolines using Formic Acid as the Hydrogen Source

      Conghui Xu, Lingjuan Zhang, Chaonan Dong, Jianbin Xu, Yixiao Pan, Yali Li, Hanyu Zhang, Huanrong Li, Zhiyong Yu and Lijin Xu

      Article first published online: 11 FEB 2016 | DOI: 10.1002/adsc.201500909

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    4. Copper-Catalyzed Coupling of Indoles with Dimethylformamide as a Methylenating Reagent

      Fan Pu, Yang Li, Yong-Hong Song, Jianliang Xiao, Zhong-Wen Liu, Chao Wang, Zhao-Tie Liu, Jian-Gang Chen and Jian Lu

      Article first published online: 11 FEB 2016 | DOI: 10.1002/adsc.201500874

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  5. Full Papers

  6. Communications

    1. Brook/Elimination/Aldol Reaction Sequence for the Direct One-Pot Preparation of Difluorinated Aldols from (Trifluoromethyl)trimethylsilane and Acylsilanes

      Mélanie Decostanzi, Jérémy Godemert, Sylvain Oudeyer, Vincent Levacher, Jean-Marc Campagne and Eric Leclerc

      Article first published online: 9 FEB 2016 | DOI: 10.1002/adsc.201500849

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    2. Copper-Mediated ortho-Arylation of Benzamides with Arylboronic Acid

      Qingwen Gui, Xiang Chen, Liang Hu, Dadian Wang, Jidan Liu and Ze Tan

      Article first published online: 9 FEB 2016 | DOI: 10.1002/adsc.201500884

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  7. Full Papers

  8. Updates

  9. Full Papers

  10. Communications

  11. Full Papers

    1. Protonated Phosphazenes: Structures and Hydrogen-Bonding Organocatalysts for Carbonyl Bond Activation

      Damien Jardel, Clotilde Davies, Frédéric Peruch, Stéphane Massip and Brigitte Bibal

      Article first published online: 4 FEB 2016 | DOI: 10.1002/adsc.201600062

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  12. Cover Pictures

    1. Towards Keratan Sulfate by Combinatorial Chemoenzymatic Synthesis of Sulfated N-Acetyllactosamine Oligomers

      Bastian Lange, Anna Šimonová, Thomas Fischöder, Helena Pelantová, Vladimír Křen and Lothar Elling

      Article first published online: 27 JAN 2016 | DOI: 10.1002/adsc.201600021

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      The cover picture, provided by Lothar Elling, Vladimir Křen, and their co-workers, illustrates the chemoenzymatic synthesis of sulfated N-acetyllactosamine (LacNAc) oligomers representing building blocks of keratan sulfate, a protein-bound glycosaminoglycan of the extracellular matrix. The modular combination of chemical sulfation and enzymatic glycan synthesis renders hexasaccharides with variable degrees of sulfation. The reported sulfated glycan structures are potential candidates for binding assays of glycan binding proteins such as lectins and growth factors. Details can be found in the full paper on pages xxxx-xxxx (B. Lange, A. Šimonová, T. Fischöder, H. Pelantová, V. Křen, L. Elling, Adv. Synth. Catal.­ 2016, 358, xxxx-xxxx; DOI: 10.1002/adsc.201500916).

  13. Communications

    1. Copper(I)-Catalysed Multicomponent Reaction: Straightforward Access to 5-Hydroxy-1H-pyrrol-2(5H)-ones

      Muhammad Idham Darussalam Mardjan, Jean-Luc Parrain and Laurent Commeiras

      Article first published online: 26 JAN 2016 | DOI: 10.1002/adsc.201500994

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    2. Asymmetric Transfer Hydrogenation of Ketones with Modified Grubbs Metathesis Catalysts: On the Way to a Tandem Process

      Marc Renom-Carrasco, Piotr Gajewski, Luca Pignataro, Johannes G. de Vries, Umberto Piarulli, Cesare Gennari and Laurent Lefort

      Article first published online: 26 JAN 2016 | DOI: 10.1002/adsc.201500933

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  14. Full Papers

    1. Very Important Publication

    2. Rhodium-Catalyzed Bis-Hydroaminomethylation of Linear Aliphatic Alkenes with Piperazine

      Thomas Seidensticker, Jonas M. Vosberg, Karoline A. Ostrowski and Andreas J. Vorholt

      Article first published online: 26 JAN 2016 | DOI: 10.1002/adsc.201500896

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    3. Very Important Publication

      A Chiral Disulfoxide Ligand for the Efficient Rhodium-Catalyzed 1,2-Addition of Arylboroxines to N-Tosylarylimines

      Guang-Zhen Zhao, Gellért Sipos, Alvaro Salvador, Arnold Ou, Pengchao Gao, Brian W. Skelton and Reto Dorta

      Article first published online: 26 JAN 2016 | DOI: 10.1002/adsc.201500975

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  15. Communications

  16. Full Papers

    1. Very Important Publication

  17. Updates

    1. Very Important Publication

    2. Improved Second Generation Iron Pincer Complexes for Effective Ester Hydrogenation

      Saravanakumar Elangovan, Bianca Wendt, Christoph Topf, Stephan Bachmann, Michelangelo Scalone, Anke Spannenberg, Haijun Jiao, Wolfgang Baumann, Kathrin Junge and Matthias Beller

      Article first published online: 22 JAN 2016 | DOI: 10.1002/adsc.201500930

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  18. Full Papers

    1. Very Important Publication

      Towards Keratan Sulfate – Chemoenzymatic Cascade Synthesis of Sulfated N-Acetyllactosamine (LacNAc) Glycan Oligomers

      Bastian Lange, Anna Šimonová, Thomas Fischöder, Helena Pelantová, Vladimír Křen and Lothar Elling

      Article first published online: 22 JAN 2016 | DOI: 10.1002/adsc.201500916

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  19. Communications

  20. Full Papers

    1. Palladium-Catalyzed [2+1] Cycloadditions Affording Vinylidenecyclopropanes as Precursors of 7-Membered Carbocycles

      Aymeric Lepronier, Thierry Achard, Laurent Giordano, Alphonse Tenaglia, Gérard Buono and Hervé Clavier

      Article first published online: 12 JAN 2016 | DOI: 10.1002/adsc.201500971

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    2. Very Important Publication

  21. Cover Pictures

    1. You have free access to this content
      Enlarged scope of direct C-H olefination

      Xiao Xue, Jianbin Xu, Lingjuan Zhang, Conghui Xu, Yixiao Pan, Lijin Xu, Huanrong Li and Weidong Zhang

      Article first published online: 5 JAN 2016 | DOI: 10.1002/adsc.201501054

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      The front cover picture, provided by Lijin Xu, Weidong Zhang and co-workers, illustrates an efficient and versatile Rh(III)-catalyzed direct ortho-olefination of arenes, such as benzamides, arylpyridines and indoles, with unactivated aliphatic olefins bearing different substitution patterns. This reaction exhibits high regio- and stereo-selectivity, functional group tolerance, and ample substrate scope. This new method expands the scope of rhodium(III)-catalyzed direct C-H bond olefination of arenes, and provides a rapid access to useful linear arylation products of unactivated aliphatic olefins. Details can be found in the full paper on pages XXXX–XXXX (X. Xue, J. Xu, L. Zhang, C. Xu, Y. Pan, L. Xu, H. Li, W. Zhang, Adv. Synth. Catal.­ 2016, 358, XXXX–XXXX; DOI: 10.1002/adsc.201500697).

  22. Full Papers

  23. Communications

    1. Very Important Publication

  24. Cover Pictures

    1. You have free access to this content
      Sequential Functionalization of O[BOND]H and C(sp2)[BOND]O Bonds from Alkynes, N-Sulfonyl Azides, and Tropolones

      Boram Seo, Woo Hyung Jeon, Chul-Eui Kim, Sanghyuck Kim, Sung Hong Kim and Phil Ho Lee

      Article first published online: 22 DEC 2015 | DOI: 10.1002/adsc.201501042

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      The front cover picture, provided by Phil Ho Lee and co-workers, illustrates Rh-catalyzed reaction of tropolones with N-tosyl-1,2,3-triazoles for the synthesis of the 2-functionalized aminotropones via tandem Rh-catalyzed O[BOND]H insertion, intramolecular 1,8-addition, and rearrangement in one pot. Sequential Cu-catalyzed [3+2] cycloaddition, Rh-catalyzed O[BOND]H insertion, intramolecular 1,8-addition, and rearrangement starting from 1-alkynes, N-sulfonyl azides, and tropolones is also described for the synthesis of the 2-functionalized aminotropones in one pot. Details can be found in the full paper on pages XXXX-XXXX (B. Seo, W. H. Jeon, C.-E. Kim, S. Kim, S. H. Kim, P. H. Lee, Adv. Synth. Catal.­ 2016, 358, XXXX–XXXX; DOI: 10.1002/adsc.201500829).

    2. You have free access to this content
      Robust Silver(I) Catalyst for the Carboxylative Cyclization of Propargylic Alcohols with Carbon Dioxide under Ambient Conditions

      Qing-Wen Song and Liang-Nian He

      Article first published online: 18 DEC 2015 | DOI: 10.1002/adsc.201501051

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      The front cover picture, provided by Qing-Wen Song and Liang-Nian He, illustrates a silver-catalyzed carboxylative cyclization of propargylic alcohols/propargylic amines with CO2 for the synthesis of α-alkylidene cyclic carbonates/oxazolidinones under ambient conditions without employing any additional organic base and ligand. The synergistic effect of Lewis basic and Lewis acidic species in conjunction with the bulkier counterion, via the alkyl carbonate intermediate, leads to the excellent efficiency. The picture shows an outline of exhaust gas and chemical conversion via a sustainable CO2 recycling process into value-added products using a green catalytic method. Details can be found in the full paper on pages xxxx–xxxx (Q.-W. Song and L.-N. He, Adv. Synth. Catal.­ 2016, 358, xxxx–xxxx; DOI: 10.1002/adsc.201500639).

  25. Full Papers

    1. Very Important Publication

    2. Sequential Functionalization of the O[BOND]H and C(sp2)[BOND]O Bonds of Tropolones by Alkynes and N-Sulfonyl Azides

      Boram Seo, Woo Hyung Jeon, Chul-Eui Kim, Sanghyuck Kim, Sung Hong Kim and Phil Ho Lee

      Article first published online: 9 DEC 2015 | DOI: 10.1002/adsc.201500829

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    3. Rhodium(III)-Catalyzed Direct C[BOND]H Olefination of Arenes with Aliphatic Olefins

      Xiao Xue, Jianbin Xu, Lingjuan Zhang, Conghui Xu, Yixiao Pan, Lijin Xu, Huanrong Li and Weidong Zhang

      Article first published online: 25 NOV 2015 | DOI: 10.1002/adsc.201500697

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