Advanced Functional Materials

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  1. Colorectal Cancer Diagnosis Using Enzyme-Sensitive Ratiometric Fluorescence Dye and Antibody–Quantum Dot Conjugates for Multiplexed Detection

    Youngrong Park, Yeon-Mi Ryu, Taejun Wang, Yebin Jung, Sohee Kim, Sekyu Hwang, Joonhyuck Park, Dong-Jun Bae, Jaeil Kim, Heejo Moon, Hyun-Suk Lim, Sang-Yeob Kim, Euiheon Chung, Ki Hean Kim, Sungjee Kim and Seung-Jae Myung

    Version of Record online: 22 NOV 2017 | DOI: 10.1002/adfm.201703450

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    A ratiometric fluorescent probe that responds to the λ-glutamyltranspeptidase activity is developed and co-used with an antibody–quantum dot conjugate probe, which demonstrates the potential for endoscopic early colon cancer diagnosis by multiplexed and complementary detection of colorectal tumors and precancerous regions such as adenoma and hyperplasia.

  2. Single Crystal Microwires of p-DTS(FBTTh2)2 and Their Use in the Fabrication of Field-Effect Transistors and Photodetectors

    Qiuhong Cui, Yuanyuan Hu, Cheng Zhou, Feng Teng, Jianfei Huang, Andriy Zhugayevych, Sergei Tretiak, Thuc-Quyen Nguyen and Guillermo C. Bazan

    Version of Record online: 22 NOV 2017 | DOI: 10.1002/adfm.201702073

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    Crystalline microwires of p-DTS(FBTTh2)2 are fabricated via solution-phase self-assembly. Such wires exhibit good charge mobility and highly photosensitive response characteristics. Furthermore, these experimental results are interpreted and rationalized using theoretical simulations.

  3. An Ultrathin Flexible 2D Membrane Based on Single-Walled Nanotube–MoS2 Hybrid Film for High-Performance Solar Steam Generation

    Xiangdong Yang, Yanbing Yang, Linna Fu, Mingchu Zou, Zhihao Li, Anyuan Cao and Quan Yuan

    Version of Record online: 22 NOV 2017 | DOI: 10.1002/adfm.201704505

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    To address the difficulties in obtaining photothermal materials with ultrathin structure yet sufficient solar spectrum absorption capability, an ultrathin and self-floating SWNT–MoS2 hybrid film is designed. As an interfacial heating membrane, this SWNT–MoS2 film shows enhanced steam generation efficiency and superior recycle stability due to the ultrathin and porous structure as well as high mechanical strength.

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    Combination of Hybrid CVD and Cation Exchange for Upscaling Cs-Substituted Mixed Cation Perovskite Solar Cells with High Efficiency and Stability

    Yan Jiang, Matthew R. Leyden, Longbin Qiu, Shenghao Wang, Luis K. Ono, Zhifang Wu, Emilio J. Juarez-Perez and Yabing Qi

    Version of Record online: 22 NOV 2017 | DOI: 10.1002/adfm.201703835

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    Cs-substituted mixed perovskite modules are prepared by a new developed large-area-compatible method combining hybrid chemical vapor deposition and cation exchange. Power conversion efficiency (PCE) as high as 14.6% is achieved, benefiting from the large-area film uniformity on macroscopic and microscopic scales. In-depth study shows that 7% Cs+ in CsxFA1−xPbI3 is the optimal ratio for achieving best device PCE and longest lifetime.

  5. Kinetically Controlled Coprecipitation for General Fast Synthesis of Sandwiched Metal Hydroxide Nanosheets/Graphene Composites toward Efficient Water Splitting

    Tang Tang, Wen-Jie Jiang, Shuai Niu, Ning Liu, Hao Luo, Qiang Zhang, Wu Wen, Yu-Yun Chen, Lin-Bo Huang, Feng Gao and Jin-Song Hu

    Version of Record online: 22 NOV 2017 | DOI: 10.1002/adfm.201704594

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    Kinetically controlled coprecipitation strategy is developed as a general cost-effective strategy to prepare sandwiched metal hydroxide/graphene nanocomposites. Nickel cobalt hydroxide nanosheets vertically assembled on graphene exhibit superior electrocatalytic activity and durability for oxygen evolution reaction, which enables the developed strategy to mass produce a variety of hydroxide/graphene nanocomposites for diverse energy applications.