© WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
Editor: Michael Rowan; Editorial Board Chairs: Uwe Bornscheuer, Luis A. Oro, Bert Weckhuysen
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ISI Journal Citation Reports © Ranking: 2015: 29/144 (Chemistry Physical)
Online ISSN: 1867-3899
March 24, 2015
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Recently Published Articles
- Ruthenium-Catalyzed Metathesis of Conjugated Polyenes
Áron Balla, Dr. Mohammed Al-Hashimi, Antisar Hlil, Prof. Hassan S. Bazzi and Dr. Robert Tuba
Version of Record online: 28 JUL 2016 | DOI: 10.1002/cctc.201600479
Metathesize it up: An understanding of the mechanism of the interconversion of ruthenium N-heterocyclic carbene η1–η3-allyl complexes may open the way for the development of a new generation of ruthenium-based latent metathesis catalyst systems. This review summarizes the most relevant pioneering work focused on conjugated polyene metathesis to lead to new ideas for the development of forthcoming metathesis catalysts in different applications.
- Selective Hydrogenation of Benzene to Cyclohexene over 2Ru/La2O3-ZnO Catalyst without Additional Modifiers
Hendrik Spod, Martin Lucas and Prof. Dr. Peter Claus
Version of Record online: 28 JUL 2016 | DOI: 10.1002/cctc.201600493
Benzene hydrogenation: A simple 2Ru/La2O3-ZnO catalyst was tested in the selective hydrogenation of benzene. The droplet size of the organic compound in the complex four-phase system (g/l/l/s) was determined for the first time in situ under the reaction conditions.
- Brønsted or Lewis Acid Initiated Multicomponent Cascade Reaction: Diastereoselective Synthesis of Imidazolidinyl Spirooxindole Derivatives
Jun-Qi Zhang, Zheng-Hang Qi, Shao-Jie Yin, Hai-Yan Li, Prof. Dr. Yong Wang and Prof. Dr. Xing-Wang Wang
Version of Record online: 28 JUL 2016 | DOI: 10.1002/cctc.201600560
Cheap but good: A three-component [2+2+1] cascade reaction of 1,4-oxazepines with diazo-oxindoles is studied theoretically and experimentally for the construction of aza-hetero-imidazolidinyl spirooxindole derivatives. The reactions are catalyzed by iron(II) trifluoromethanesulfonate and p-toluenesulfonic acid monohydrate, respectively, giving high yields with excellent diastereoselectivity.
- In situ Integration of a Metallic 1T-MoS2/CdS Heterostructure as a means To Promote Visible-Light-Driven Photocatalytic Hydrogen Evolution
Qin Liu, Qichao Shang, Adnan Khalil, Qi Fang, Shuangming Chen, Qun He, Ting Xiang, Daobin Liu, Prof. Qun Zhang, Prof. Yi Luo and Prof. Li Song
Version of Record online: 28 JUL 2016 | DOI: 10.1002/cctc.201600504
Grow up! Undesirable electron–hole recombination of CdS nanorods is significantly suppressed by a facile solvothermal method involving the in situ growth of few-layered 1T-MoS2 slabs. This brings about a dramatic enhancement in the photocatalytic performance. In situ growth of a 1T heterojunction is thus a new pathway to boost photo/electrocatalytic properties.
- Suppression of the Aromatic Cycle in Methanol-to-Olefins Reaction over ZSM-5 by Post-Synthetic Modification Using Calcium
Irina Yarulina, Simon Bailleul, Alexey Pustovarenko, Dr. Javier Ruiz Martinez, Dr. Kristof De Wispelaere, Julianna Hajek, Prof. Dr. Bert M. Weckhuysen, Dr. Klaartje Houben, Prof. Dr. Marc Baldus, Prof. Dr. Veronique Van Speybroeck, Prof. Dr. Freek Kapteijn and Prof. Dr. Jorge Gascon
Version of Record online: 28 JUL 2016 | DOI: 10.1002/cctc.201600650
Calcium against aromatics: The incorporation of Ca in ZSM-5 results in a 90 percent selectivity towards light olefins, and a nine times longer catalyst lifetime in the methanol-to-olefins reaction. Theoretical calculations point to the formation of CaOCaOH+, which weakens the acid strength of the zeolite, resulting in the suppression of the aromatic cycle.