The full text of this article hosted at iucr.org is unavailable due to technical difficulties.

Zuschrift

Nanostructure Engineering and Doping of Conjugated Carbon Nitride Semiconductors for Hydrogen Photosynthesis

Zhenzhen Lin

Research Institute of Photocatalysis, Fujian Provincial Key Laboratory of Photocatalysis‐State Key Laboratory Breeding Base, and College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002 (China)

Search for more papers by this author
Prof. Xinchen Wang

Corresponding Author

E-mail address: xcwang@fzu.edu.cn

Research Institute of Photocatalysis, Fujian Provincial Key Laboratory of Photocatalysis‐State Key Laboratory Breeding Base, and College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002 (China)

Research Institute of Photocatalysis, Fujian Provincial Key Laboratory of Photocatalysis‐State Key Laboratory Breeding Base, and College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002 (China)
Search for more papers by this author
First published: 07 January 2013
Cited by: 90

Supported by the National Basic Research Program of China (2013CB632405), the National Natural Science Foundation of China (21033003, 21173043), and the Department of Education of Fujian Province in China. The authors appreciate Prof. L. Li of Xiamen University (China) for the AFM measurements.

Abstract

Optimiert: Die simultane Modifizierung der Bulk‐, Oberflächen‐ und elektronischen Struktur eines Kohlenstoffnitridpolymers gelang durch direkte Cokondensation von Harnstoff und Ph4BNa. Mit diesem Verfahren werden bordotierte Kohlenstoffnitridnanoblätter erhalten (siehe Bild), die den Lichteinfang optimieren und die Oberflächenreaktivität bei der Wasserstoffphotosynthese erhöhen.

Number of times cited according to CrossRef: 90

  • , Cost‐Efficient Graphitic Carbon Nitride as an Effective Photocatalyst for Antibiotic Degradation: An Insight into the Effects of Different Precursors and Coexisting Ions, and Photocatalytic Mechanism, Chemistry – An Asian Journal, 14, 1, (162-169), (2018).
  • , Achieving Efficient Incorporation of π‐Electrons into Graphitic Carbon Nitride for Markedly Improved Hydrogen Generation, Angewandte Chemie International Edition, 58, 7, (1985-1989), (2019).
  • , Achieving Efficient Incorporation of π‐Electrons into Graphitic Carbon Nitride for Markedly Improved Hydrogen Generation, Angewandte Chemie, 131, 7, (2007-2011), (2019).
  • , Tuning Nitrogen Content in Carbon Nitride by Isonicotinic Acid for Highly Efficient Photocatalytic Hydrogen Evolution, ChemCatChem, 11, 3, (1045-1056), (2019).
  • , Mesoporous graphitic carbon nitride (g-C 3 N 4 ) nanosheets synthesized from carbonated beverage-reformed commercial melamine for enhanced photocatalytic hydrogen evolution , Materials Chemistry Frontiers, 10.1039/C8QM00577J, (2019).
  • , Powerful combination of MOFs and C3N4 for enhanced photocatalytic performance, Applied Catalysis B: Environmental, 10.1016/j.apcatb.2019.01.091, (2019).
  • , Carbon Vacancies in a Melon Polymeric Matrix Promote Photocatalytic Carbon Dioxide Conversion, Angewandte Chemie International Edition, 58, 4, (1134-1137), (2018).
  • , Carbon Vacancies in a Melon Polymeric Matrix Promote Photocatalytic Carbon Dioxide Conversion, Angewandte Chemie, 131, 4, (1146-1149), (2018).
  • , Fabrication of Tubular g‐C3N4 with N‐Defects and Extended π‐Conjugated System for Promoted Photocatalytic Hydrogen Production, ChemCatChem, 11, 5, (1534-1544), (2019).
  • , Oligomer‐Incorporated Polymeric Layer Framework of Graphitic Carbon Nitride for Effective Photocatalytic Hydrogen Evolution, Particle & Particle Systems Characterization, 35, 1, (2017).
  • , Organosilica Nanotube Templates: One‐Pot Synthesis of Carbon‐Modified Polymeric Carbon Nitride Nanorods for Photocatalysis, ChemCatChem, 10, 3, (581-589), (2017).
  • , Heteroatom‐Doped Carbonaceous Photocatalysts for Solar Fuel Production and Environmental Remediation, ChemCatChem, 10, 1, (62-123), (2017).
  • , WS2/Graphitic Carbon Nitride Heterojunction Nanosheets Decorated with CdS Quantum Dots for Photocatalytic Hydrogen Production, ChemSusChem, 11, 7, (1187-1197), (2018).
  • , Embedding Carbon Nitride into a Covalent Organic Framework with Enhanced Photocatalysis Performance, Chemistry – An Asian Journal, 13, 13, (1674-1677), (2018).
  • , Biomimetic Donor–Acceptor Motifs in Conjugated Polymers for Promoting Exciton Splitting and Charge Separation, Angewandte Chemie, 130, 28, (8865-8869), (2018).
  • , Biomimetic Donor–Acceptor Motifs in Conjugated Polymers for Promoting Exciton Splitting and Charge Separation, Angewandte Chemie International Edition, 57, 28, (8729-8733), (2018).
  • , Fluorescent Sulphur‐ and Nitrogen‐Containing Porous Polymers with Tuneable Donor–Acceptor Domains for Light‐Driven Hydrogen Evolution, Chemistry – A European Journal, 24, 46, (11916-11921), (2018).
  • , Triamterene‐Grafted Graphitic Carbon Nitride with Electronic Potential Redistribution for Efficient Photocatalytic Hydrogen Evolution, Chemistry – An Asian Journal, 13, 20, (3073-3083), (2018).
  • , Ni-Mo nanoparticles as co-catalyst for drastically enhanced photocatalytic hydrogen production activity over g-C3N4, Applied Catalysis B: Environmental, 10.1016/j.apcatb.2018.10.003, (2018).
  • , Fluorine Modified Boron Carbon Nitride Semiconductors for Improved Photocatalytic CO2 Reduction under Visible Light, ChemCatChem, 10, 22, (5270-5279), (2018).
  • , g‐C3N4 Inverse Opals with Isotype Heterostructure for Enhanced Visible‐Light‐Driven Photocatalysis, Chemistry – An Asian Journal, 13, 21, (3261-3267), (2018).
  • , Graphitic carbon nitride (g-C 3 N 4 ) electrodes for energy conversion and storage: a review on photoelectrochemical water splitting, solar cells and supercapacitors , Journal of Materials Chemistry A, 10.1039/C8TA08001A, (2018).
  • , Integrating MoS2 on sulfur-doped porous g-C3N4 iostype heterojunction hybrids enhances visible-light photocatalytic performance, Journal of Alloys and Compounds, 10.1016/j.jallcom.2018.07.286, 768, (766-774), (2018).
  • , Construction of 2D-composite HCa 2 Nb 3 O 10 /CaNb 2 O 6 heterostructured photocatalysts with enhanced hydrogen production performance , New Journal of Chemistry, 10.1039/C7NJ03707D, 42, 1, (681-687), (2018).
  • , Amino‐Assisted Anchoring of CsPbBr3 Perovskite Quantum Dots on Porous g‐C3N4 for Enhanced Photocatalytic CO2 Reduction, Angewandte Chemie, 130, 41, (13758-13762), (2018).
  • , Amino‐Assisted Anchoring of CsPbBr3 Perovskite Quantum Dots on Porous g‐C3N4 for Enhanced Photocatalytic CO2 Reduction, Angewandte Chemie International Edition, 57, 41, (13570-13574), (2018).
  • , Optimizing Optical Absorption, Exciton Dissociation, and Charge Transfer of a Polymeric Carbon Nitride with Ultrahigh Solar Hydrogen Production Activity, Angewandte Chemie International Edition, 56, 43, (13445-13449), (2017).
  • , Optimizing Optical Absorption, Exciton Dissociation, and Charge Transfer of a Polymeric Carbon Nitride with Ultrahigh Solar Hydrogen Production Activity, Angewandte Chemie, 129, 43, (13630-13634), (2017).
  • , From Millimeter to Subnanometer: Vapor–Solid Deposition of Carbon Nitride Hierarchical Nanostructures Directed by Supramolecular Assembly, Angewandte Chemie, 129, 29, (8546-8550), (2017).
  • , From Millimeter to Subnanometer: Vapor–Solid Deposition of Carbon Nitride Hierarchical Nanostructures Directed by Supramolecular Assembly, Angewandte Chemie International Edition, 56, 29, (8426-8430), (2017).
  • , Metal‐Free Boron‐Containing Heterogeneous Catalysts, Angewandte Chemie International Edition, 56, 49, (15506-15518), (2017).
  • , , Angewandte Chemie, 129, 49, (15712-15724), (2017).
  • , Enhanced Separation Efficiency of PtNi/g‐C3N4 for Photocatalytic Hydrogen Production, ChemCatChem, 9, 19, (3779-3785), (2017).
  • , C=C π Bond Modified Graphitic Carbon Nitride Films for Enhanced Photoelectrochemical Cell Performance, Chemistry – An Asian Journal, 12, 9, (1005-1012), (2017).
  • , Synthesis of Layered Carbonitrides from Biotic Molecules for Photoredox Transformations, Angewandte Chemie International Edition, 56, 23, (6627-6631), (2017).
  • , Synthesis of Layered Carbonitrides from Biotic Molecules for Photoredox Transformations, Angewandte Chemie, 129, 23, (6727-6731), (2017).
  • , Strategies for Efficient Solar Water Splitting Using Carbon Nitride, Chemistry – An Asian Journal, 12, 13, (1421-1434), (2017).
  • , A Continuous Carbon Nitride Polyhedron Assembly for High‐Performance Flexible Supercapacitors, Advanced Functional Materials, 27, 8, (2017).
  • , A three-dimensional graphitic carbon nitride belt network for enhanced visible light photocatalytic hydrogen evolution, J. Mater. Chem. A, 10.1039/C6TA07397B, 4, 48, (19003-19010), (2016).
  • , Construction of a magnetic Z-scheme photocatalyst with enhanced oxidation/reduction abilities and recyclability for the degradation of tetracycline, RSC Advances, 6, 115, (114374), (2016).
  • , Conjugated Polymers: Catalysts for Photocatalytic Hydrogen Evolution, Angewandte Chemie International Edition, 55, 51, (15712-15727), (2016).
  • , Water Compatible Conjugated Microporous Polyazulene Networks as Visible‐Light Photocatalysts in Aqueous Medium, ChemCatChem, 8, 4, (694-698), (2016).
  • , Construction of Large‐Scale Ultrathin Graphitic Carbon Nitride Nanosheets by a Hydrogen‐Bond‐Assisted Strategy for Improved Photocatalytic Hydrogen Production and Ciprofloxacin Degradation Activity, ChemCatChem, 8, 17, (2838-2845), (2016).
  • , Homogenous Boron‐doping in Self‐sensitized Carbon Nitride for Enhanced Visible‐light Photocatalytic Activity, Chemistry – An Asian Journal, 11, 22, (3169-3173), (2016).
  • , A Rapid Microwave‐Assisted Thermolysis Route to Highly Crystalline Carbon Nitrides for Efficient Hydrogen Generation, Angewandte Chemie, 128, 47, (14913-14917), (2016).
  • , Graphitic Carbon Nitride/Nitrogen‐Rich Carbon Nanofibers: Highly Efficient Photocatalytic Hydrogen Evolution without Cocatalysts, Angewandte Chemie, 128, 36, (11007-11011), (2016).
  • , Graphitic Carbon Nitride/Nitrogen‐Rich Carbon Nanofibers: Highly Efficient Photocatalytic Hydrogen Evolution without Cocatalysts, Angewandte Chemie International Edition, 55, 36, (10849-10853), (2016).
  • , Facile Construction of g‐C3N4 Nanosheets/TiO2 Nanotube Arrays as Z‐Scheme Photocatalyst with Enhanced Visible‐Light Performance, ChemCatChem, 8, 19, (3064-3073), (2016).
  • , Hydrogen from Water over Openly‐Structured Graphitic Carbon Nitride Polymer through Photocatalysis, ChemSusChem, 9, 5, (478-484), (2016).
  • , Graphitic Carbon Nitride Film: An Emerging Star for Catalytic and Optoelectronic Applications, ChemSusChem, 9, 19, (2723-2735), (2016).
  • , , Angewandte Chemie, 128, 51, (15940-15956), (2016).
  • , A Rapid Microwave‐Assisted Thermolysis Route to Highly Crystalline Carbon Nitrides for Efficient Hydrogen Generation, Angewandte Chemie International Edition, 55, 47, (14693-14697), (2016).
  • , Protic Salts of High Nitrogen Content as Versatile Precursors for Graphitic Carbon Nitride: Anion Effect on the Structure, Properties, and Photocatalytic Activity, ChemPlusChem, 80, 7, (1139-1147), (2015).
  • , Photocatalytic Hydrogen Evolution from Silica‐Templated Polymeric Graphitic Carbon Nitride–Is the Surface Area Important?, ChemCatChem, 7, 1, (121-126), (2014).
  • , Conjugated Microporous Poly(Benzochalcogenadiazole)s for Photocatalytic Oxidative Coupling of Amines under Visible Light, ChemSusChem, 8, 20, (3459-3464), (2015).
  • , Heterophase Photocatalysts from Water‐Soluble Conjugated Polyelectrolytes: An Example of Self‐Initiation under Visible Light, Angewandte Chemie International Edition, 54, 48, (14549-14553), (2015).
  • , Graphitic Carbon Nitride Polymers toward Sustainable Photoredox Catalysis, Angewandte Chemie International Edition, 54, 44, (12868-12884), (2015).
  • , Phosphorus‐Doped Graphitic Carbon Nitrides Grown In Situ on Carbon‐Fiber Paper: Flexible and Reversible Oxygen Electrodes, Angewandte Chemie International Edition, 54, 15, (4646-4650), (2014).
  • , Heterophasen‐Photokatalysatoren aus wasserlöslichen Polyelektrolyten: ein Beispiel für die Selbstinitiierung unter sichtbarem Licht, Angewandte Chemie, 127, 48, (14757-14761), (2015).
  • , A Graphitic‐C3N4 “Seaweed” Architecture for Enhanced Hydrogen Evolution, Angewandte Chemie, 127, 39, (11595-11599), (2015).
  • , Merging Surface Organometallic Chemistry with Graphitic Carbon Nitride Photocatalysis for CO2 Photofixation, ChemCatChem, 7, 9, (1422-1423), (2015).
  • , Facile Synthesis and Enhanced Visible‐Light Photocatalysis of Graphitic Carbon Nitride Composite Semiconductors, ChemSusChem, 8, 7, (1189-1196), (2015).
  • , Carbon Nanosheets: Synthesis and Application, ChemSusChem, 8, 12, (2004-2027), (2015).
  • , Corrosion‐Mediated Self‐Assembly (CMSA): Direct Writing Towards Sculpturing of 3D Tunable Functional Nanostructures, Angewandte Chemie International Edition, 54, 52, (15804-15808), (2015).
  • , A Graphitic‐C3N4 “Seaweed” Architecture for Enhanced Hydrogen Evolution, Angewandte Chemie International Edition, 54, 39, (11433-11437), (2015).
  • , Corrosion‐Mediated Self‐Assembly (CMSA): Direct Writing Towards Sculpturing of 3D Tunable Functional Nanostructures, Angewandte Chemie, 127, 52, (16030-16034), (2015).
  • , Polymeres graphitisches Kohlenstoffnitrid für die nachhaltige Photoredoxkatalyse, Angewandte Chemie, 127, 44, (13060-13077), (2015).
  • , Phosphorus‐Doped Graphitic Carbon Nitrides Grown In Situ on Carbon‐Fiber Paper: Flexible and Reversible Oxygen Electrodes, Angewandte Chemie, 127, 15, (4729-4733), (2014).
  • , Noble‐Metal‐Free Molybdenum Disulfide Cocatalyst for Photocatalytic Hydrogen Production, ChemSusChem, 8, 24, (4113-4127), (2015).
  • , Facile Synthesis of Crystalline Polymeric Carbon Nitrides with an Enhanced Photocatalytic Performance under Visible Light, ChemCatChem, 7, 18, (2897-2902), (2015).
  • , Surface Modification of Carbon Nitride Polymers by Core–Shell Nickel/Nickel Oxide Cocatalysts for Hydrogen Evolution Photocatalysis, ChemCatChem, 7, 18, (2864-2870), (2015).
  • , Harvesting Solar Light with Crystalline Carbon Nitrides for Efficient Photocatalytic Hydrogen Evolution, Angewandte Chemie, 126, 41, (11181-11185), (2014).
  • , Harvesting Solar Light with Crystalline Carbon Nitrides for Efficient Photocatalytic Hydrogen Evolution, Angewandte Chemie International Edition, 53, 41, (11001-11005), (2014).
  • , Multifunctional Porous Microspheres Based on Peptide–Porphyrin Hierarchical Co‐Assembly, Angewandte Chemie International Edition, 53, 9, (2366-2370), (2014).
  • , Fabrication of H3PW12O40-doped carbon nitride nanotubes by one-step hydrothermal treatment strategy and their efficient visible-light photocatalytic activity toward representative aqueous persistent organic pollutants degradation, Applied Catalysis B: Environmental, 10.1016/j.apcatb.2014.03.010, 156-157, (141-152), (2014).
  • , Synthesis of Potassium‐Modified Graphitic Carbon Nitride with High Photocatalytic Activity for Hydrogen Evolution, ChemSusChem, 7, 9, (2654-2658), (2014).
  • , Perovskite Oxide Nanosheets with Tunable Band‐Edge Potentials and High Photocatalytic Hydrogen‐Evolution Activity, Angewandte Chemie International Edition, 53, 48, (13164-13168), (2014).
  • , Helical Graphitic Carbon Nitrides with Photocatalytic and Optical Activities, Angewandte Chemie, 126, 44, (12120-12124), (2014).
  • , Helical Graphitic Carbon Nitrides with Photocatalytic and Optical Activities, Angewandte Chemie International Edition, 53, 44, (11926-11930), (2014).
  • , Perovskite Oxide Nanosheets with Tunable Band‐Edge Potentials and High Photocatalytic Hydrogen‐Evolution Activity, Angewandte Chemie, 126, 48, (13380-13384), (2014).
  • , Multifunctional Porous Microspheres Based on Peptide–Porphyrin Hierarchical Co‐Assembly, Angewandte Chemie, 126, 9, (2398-2402), (2014).
  • , Layered Nanojunctions for Hydrogen‐Evolution Catalysis, Angewandte Chemie International Edition, 52, 13, (3621-3625), (2013).
  • , Xinchen Wang, Angewandte Chemie International Edition, 52, 37, (9610-9610), (2013).
  • , Layered Nanojunctions for Hydrogen‐Evolution Catalysis, Angewandte Chemie, 125, 13, (3709-3713), (2013).
  • , Xinchen Wang, Angewandte Chemie, 125, 37, (9788-9788), (2013).
  • , LiCl as Phase‐Transfer Catalysts to Synthesize Thin Co2P Nanosheets for Oxygen Evolution Reaction, ChemSusChem, , (2018).
  • , Polydopamine and Barbituric Acid Co‐Modified Carbon Nitride Nanospheres for Highly Active and Selective Photocatalytic CO2 Reduction, European Journal of Inorganic Chemistry, , (2018).
  • , An Effective Approach to Improve the Photocatalytic Activity of Graphitic Carbon Nitride via Hydroxyl Surface Modification, Catalysts, 10.3390/catal9010017, 9, 1, (17), (2018).
  • , Crystalline Carbon Nitride Semiconductors for Photocatalytic Water Splitting, Angewandte Chemie International Edition, , (2019).
  • , Crystalline Carbon Nitride Semiconductors for Photocatalytic Water Splitting, Angewandte Chemie, , (2019).