Estimation of Atmospheric PM10 Concentration in China Using an Interpretable Deep Learning Model and Top‐of‐the‐Atmosphere Reflectance Data From China’s New Generation Geostationary Meteorological Satellite, FY‐4A

The rapid urbanization in China and the long‐range transport dust (LRTD) from arid and semi‐arid areas has resulted in an increase of PM10 concentration. In this study, an interpretable deep learning model [deep forest (DF)] with FY‐4A top‐of‐the‐atmosphere reflectance (TOAR) data were used to obtain the hourly PM10 in China. The optimal hourly average R2 of 10‐fold cross validation can achieve 0.85 (13:00 Beijing time); The R2 (RMSE, μg/m³) of the daily, monthly, and annual averages were 0.82 (24.16), 0.97 (6.53), and 0.99 (2.30), respectively. Using TOAR data, the DF model performed better than other machine learning models. The feature importance of the TOAR‐PM10 model showed that TOAR and meteorological elements both contributed significantly to the model. In spring, the PM10 in northern China was greater than that in southern China, which may be related to the LRTD. Excluding the dust weather periods, the areas with high PM10 values in China were mainly in cities and their suburbs, where were correlated with human activities. During a dust weather process, LRTD increased PM10 in northern China by 80.4%. During a mixture haze and dust weather process, the PM10 increased by 130.2% in northern China, of which LRTD led to an increase of 73.7%. The sources (from the Taklimakan Desert in China) and transmission paths of these two LRTD processes were similar. The contribution of LRTD to PM10 was related to dust intensity and meteorological conditions. The results showed that LRTD and local pollution to PM10 was both important in haze periods.

estimated the PM 10 concentration in China in the past decade.  used the space-time extremely randomized trees (STET) to generate PM10 data in China from 2015 to 2019, with a spatial resolution of 1 km, and pointed out that PM 10 showed a significant downward trend. In addition, researchers have shown the relationship between AOD and particulate matter of polar orbiting satellites in China, such as MODIS (X. Wang et al., 2020), Visible Infrared Imaging Radiometer Suite (VIIRS; Wu et al., 2016), MISR (X. Meng et al., 2018), and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP; Chen, Song, Pan, & Huang, 2022).
Polar orbiting satellites cannot obtain high time resolution data; however, the time resolution of second-generation geostationary satellites is ∼15 min with a fine spatial resolution. Recently, some studies have begun to use geostationary satellites to obtain particle concentrations (W. Wang et al., 2017;Wei et al., 2019). Previously, the geostationary satellite AOD was principally used for PM 2.5 remote sensing (J. Z. Zhang et al., 2019). The inversion of PM 10 was initiated in the 2 yr prior to this work. The geographically weighted region models and AOD of the Indian geostationary satellite (INSAT-3D) were used to estimate PM 10 . The R 2 values of the pre-, post-, and winter models were 0.624, 0.718, and 0.633, respectively (Gupta et al., 2021). The AOD data from the Geostationary Ocean Color Imager (GOCI) of the Korean geostationary satellite (GEO-KOMPASAT 2B) was used to estimate the PM 10 concentration based on two machine learning models [gradient boosted regression trees and light gradient boosting machine (LightGBM)]. The models achieved R 2 as high as 0.82 (S. Park et al., 2021). The hourly PM 10 atmospheric concentrations in China were estimated using a deep learning algorithm and the AOD data from the Japanese geostationary satellite (Himawari-8). The hourly cross validation R 2 estimated by the AOD-PM 10 model ranged from 0.82 to 0.88. The R 2 for daily, monthly, seasonal, and annual averages of atmospheric PM 10 concentrations were 0.87, 0.91, 0.94, and 0.94, respectively (Chen, Song, Shi, & Li, 2022).
The particle concentration can be effectively estimated using the AOD (Stafoggia et al., 2019). Because AOD was only provided under optimal conditions, there were a large number of missing values (Y. Park et al., 2020). The coverage of satellite top-of-the-atmosphere reflectance (TOAR) was higher than that of AOD, so TOAR was used to directly obtain the particle concentration (L. . Using the TOAR of Himawari-8 and the random forest model, the PM 2.5 , of the Yangtze River Delta (YRD) in 2016 was obtained, and the 10-fold cross validation (R 2 ) was 0.75 . Using the TOAR of the Himawari-8 and LightGBM models, the R 2 of the PM 2.5 model was 0.86 . Using TOAR directly increases the effective coverage, and the performance of the model is also very positive.
Since the Himawari-8 satellite cannot cover Xinjiang, China (Song et al., 2021;Wei, Li, Pinker, et al., 2021), China's second-generation geostationary meteorological satellite FY-4A successfully launched on 11 December 2016, can cover the entire territory of China. Its Advanced Geosynchronous Radiation Imager (AGRI) imager can provide multi-band full-disk images with a time resolution of 15 min (Y. Mao et al., 2021;Zhang, Zhu, et al., 2019). As dust is an important component of PM 10 , the Taklimakan Desert in Xinjiang, China is an important source of dust in East Asia. Using the FY-4A satellite was advantageous in estimating the contribution of dust weather to PM 10 in East Asia (B. Chen et al., 2010). At the same time, there have been no studies on estimating PM 10 from the FY-4A satellite. This study used the FY-4A satellite to estimate China's high spatial-temporal resolution for atmospheric PM 10 concentrations.
Most studies have shown that nonlinear machine-learning models can more effectively obtain the particle concentration (Paschalidou et al., 2011;Qin et al., 2018;Yin et al., 2021). This study used a deep learning model, the deep forest (DF) model (Zhou & Feng, 2017), which has the structure of a deep neural network (DNN), and replaced DNN neurons with decision tree (DT) models. Combining the advantages of the DNN and DT models, the DF model can better fit nonlinear data and provide the importance of model features to result in a more interpretable deep learning model. The hourly PM 10 concentrations in China from June 2018 to May 2019 were obtained using the DF model, FY-4A TOAR, meteorological parameters, and geographic information data. Using the results of the FY-4A TOAR-PM 10 model, the contribution of long-range transport dust (LRTD) originating in the Taklimakan Desert to atmospheric PM 10 concentrations in China and northern China was evaluated.

FY-4A TOAR Data
FY-4A is China's second-generation geostationary meteorological satellite. It contains four advanced instruments: the AGRI, the Geosynchronous Interferometric Infrared Sounder, Lightning Mapping Imager, and Space

PM 10 Data and Auxiliary Data
The hourly atmospheric PM 10 observation data were obtained from the China Environmental Monitoring Center (CEMC; China, 2012). Figure S1 in Supporting Information S1 showed the distribution of the 1,641 CEMC ground PM 10 stations. The box in the figure shows six typical urban agglomerations in China: the Guanzhong Plain (GZP), Pearl River Delta (PRD), Central China (CC), Beijing-Tianjin-Hebei (BTH), Sichuan Basin (SCB), and Yangtze River Delta (YRD).
Auxiliary data include meteorological parameters, geographic information, and time variables. Previous studies have shown that meteorological parameters and geographic information have an impact on pollutant transmission and accumulation of pollutants (Fu et al., 2008;Gao et al., 2016;Sun et al., 2016). Meteorological parameters include boundary layer height (BLH, m;Han et al., 2018), 2 m air temperature (TM, K; Ma et al., 2021), relative humidity (RH, %; F. , u and v components of 10 m wind (U10, V10, m/s; B. , and surface air pressure (SP, Pa; G. . These data were obtained from ERA-5 ECMWF reanalysis data (https://cds.climate.copernicus.eu/cdsapp#!/dataset/reanalysis-era5-land). The temporal resolution of per hour and a spatial resolution of 0.25° × 0.25° or 0.1° × 0.1° (Table 2 for   The time variable (TIME) refers to the hour difference between the current time and 0:00 on 1 January 1900. The data used in the model are listed in Table S1 in Supporting Information S1. Zhou and Feng (2017) proposed the DF model, which uses an extreme tree (ET; Geurts et al., 2006) and random forest (RF; Breiman, 2001) as neurons of the model, and multiple neurons formed a hidden layer. The DF model includes N hidden layers, and the output of the last hidden layer is connected to a separate estimator LightGBM (Ke et al., 2017) to output the results of the model. Because the DF model neurons were tree models (such as RF and ET), the DF model can output the importance of features, which makes the DF model interpretable. In this study, a DF model with three hidden layers was designed. Each layer contained 12 neurons (6 ETs and 6 RFs). Figure 1 is a structural diagram of the PM 10 concentration obtained by the DF model.

Data Preprocessing
The spatial resolution of meteorological elements and geographic information was adjusted to 0.04° × 0.04° of FY-4A data by bilinear interpolation. The PM 10 hourly mean data of CEMC were compared with those of the TOAR of FY-4A. After data matching, the total number of samples was 937,974, of which the number of samples in spring (MAM), summer (JJA), autumn (SON), and winter (DJF) were 229,769, 259,037, 300,717, and 148,451, respectively.

Model Validation
A 10-fold cross-validation method was used to test the model performance (Rodriguez et al., 2010). The parameters used to describe the model performance included the determination coefficient (R 2 ), root mean square error (RMSE), and mean absolute error (MAE; Chen, Song, Pan, & Huang, 2022;Chen, Song, Shi, & Li, 2022). The expected error (EE, Equation 1) was used to evaluate the accuracy of the TOAR-PM 10 model. The better EE value (close to 100%) indicated that the estimated value of the model is agree with the observation value (Chu et al., 2003;.
represents the observed value of PM 10 from CEMC.

Time Scale Results (Hourly, Daily, Monthly, Seasonal, and Annual Mean)
The TOAR-PM 10 model was established using the DF model, and the estimated atmospheric PM 10 concentration values were compared with the observed values of the CEMC. The results were shown in Figure 2. Except at 09:00 a.m. Beijing time, the 10-fold cross validation R 2 was greater than 0.8. At 13:00, the R 2 value of the model reached a maximum of 0.85, and 55% of the samples fell within EE. The fitting slope comparing the estimated value and the observed value was >0.8, indicating that the TOAR-PM 10 model estimated most atmospheric PM 10 samples well, and the estimated value was consistent with the observed value. The RMSE of the model was 18.44-34.72 µg/m 3 with a MAE is 10.91-16.92 µg/m 3 . This showed that it was feasible to directly obtain PM 10 concentration data using FY-4A TOAR data, and the model performance was mainly related to pollutant  . As shown in Figure 2 (I), the R 2 of the out-of-station cross validation results was 0.66, which was worse than the data based on grid points. This was because some stations did not participate in the training data of the model, so that the model could not obtain the effective information of the region. In general, considering the overall performance of the model, the DF model could effectively estimate the PM10 concentration in the area without sites.
As shown in Figures 3a-3d, the TOAR-PM 10 estimation model performed best in autumn with a cross validation R 2 was 0.84 (RMSE was 21.66 µg/m 3 ). Performance was poor during summer R 2 with a value of only 0.66 (RMSE was 22.57 µg/m 3 ). R 2 in spring and winter were 0.75 and 0.83, respectively; however, RMSE in these two seasons was relatively high, 27.19 and 29.04 µg/m 3 , respectively. This may be related to the frequent occurrence of dust weather in spring and the large combustion of fossil fuels for heating in winter (Xiao et al., 2015;. In addition, the estimated atmospheric PM 10 concentrations was compared with station observations on daily, monthly, seasonal, and annual average PM 10 . The results were shown in Figures 3e-3h. The daily, monthly, seasonal, and annual validation results R 2 (RMSE) of TOAR-PM 10 model were 0.82 (24.16 µg/m 3 ), 0.97 (6.53 µg/m 3 ), 0.98 (4.17 µg/m 3 ), and 0.99 (2.30 µg/m 3 ), respectively. The results showed that the PM 10 estimated using the TOAR-PM 10 model was reliable. Figure 4 showed the spatial performance of the TOAR-PM 10 model.  in urban agglomeration areas, and performed poorly, mainly in areas with complex topographic conditions, such as the western Sichuan Basin.

Importance of Model Features
The deep learning DNN model is a "black box," which cannot provide interpretability to the model. The neuron of the deep learning DF model is a tree model, which can obtain the importance of model features and the contribution of model input variables. To evaluate the importance of each input feature in different seasons (or regions), we used the same DF architecture (as described in Section 2.3) and retrained the data in seasons (or regions) to obtain the feature importance. Except for Figure 5a (spring, summer, autumn, and winter) and Figure 5b, the other results of the model in this article were the results of the same TOAR-PM 10 model constructed based on the whole sample, such as Figure 5a (Annual).
As shown in Figure 5a, the feature importance of TOAR (the sum of the feature importance of the four channels) was the highest, followed by the TIME variable. Among the meteorological elements, BLH, RH, and TM made significant contributions to the model. In addition, a low vegetation index (LL) also affected the performance of the model. Generally speaking, the feature importance of each input was different in seasons, but in the season with poor model performance, the contribution of other importance features was low except for TOAR. Figure 6 showed the variation trend of uncertainty (RMSE) with important features. The results indicate that the uncertainty of derived PM 10 varies with TOAR and meteorological elements. In general, various factors (including TOA and meteorological factors) influence the uncertainty of derived PM 10 . RMSE decreased with the increase of VIS_B, VIS_G, VIS_R, BLH, and TM. The effect of NIR and RH on RMSE was about 20 µg/m 3 . Furthermore, based on the feature importance, the main influencing factors of each region will change. In addition, we performed linear fitting for each estimation factor and model bias, and the regression coefficient obtained is shown in Figure S2 in Supporting Information S1. The results indicated that the factors such as VIS_G, VIS_R, RH, LL, SP, TM, and height contributed more (absolute value of the regression coefficient >1) to the uncertainty of the estimation results.
In addition, as shown in Figure 5b, the feature importance of TOAR in each region was ∼0.15, while meteorological elements, geographic information, and time variables changed significantly. BLH and RH had a significant impact on the BTH region, but their contributions to other regions were relatively low. The contribution of TM to

Spatial Distribution of Hourly and Seasonal Average for Atmospheric PM 10 Concentrations
The average PM 10 concentration distribution from 09:00 to 16:00 Beijing during the study period was shown in Figure 7. The estimation results of TOAR-PM 10 showed that the Tarim Basin had the highest concentration of atmospheric PM 10 concentration in China, with a daily average concentration of 100 µg/m3, which is correlated with frequent local dust aerosols. The concentration of PM 10 in BTH region showed obvious diurnal variation: it was the greatest from 09:00 to 10:00 (73.15 ± 22.81 µg/m 3 ), then decreased to 56.22 ± 9.87 µg/m 3 at 13:00. At 16:00 it increased slightly (63.03 ± 13.71 µg/m 3 ). The PM 10 concentration in GZP had the same diurnal variation as that in the BTH area (61.10 ± 19.96 µg/m 3 , 55.87 ± 10.98 µg/m 3 , and 58.01 ± 12.53 µg/m 3 ). The concentration of PM 10 in southern China continued to decline from 09:00 to 16:00, but there were great differences among regions: the concentration of PM 10 in the YRD region was 65 µg/m 3 and greater; The hourly variation range of PM10 concentration in CC region was 60.38 ± 17.53 µg/m 3 ; The hourly PM10 of SCB region was 53.22 ± 11.25 µg/m 3 ; The concentration of atmospheric PM 10 in the YRD region was less than 50 µg/m 3 . In addition, the concentration of PM 10 in other parts of China was relatively low, especially in Northeast China and the Qinghai Tibet Plateau. The results indicated that the estimated results were in good agreement with the observed results.
As shown in Figure S3 in Supporting Information S1, the average atmospheric PM 10 concentration values during the four seasons in China were 67.90 ± 25.78 , 49.8 ± 20.06 , 58.68 ± 22.16, and 73.46 ± 26.27 µg/m 3 , respectively. Because of the frequent dust weather in spring, the atmospheric PM 10 concentration in the Tarim Basin, one of the dust sources in East Asia, was very high, and the PM 10 concentration in North China was generally greater than that in South China. In winter, due to low wind speeds, meteorological conditions were not conducive to pollutant diffusion. Winter is the heating season in northern China. The PM 10 concentrations in the BTH, GZP, YRD, and SCB regions were greater in winter. Compared with those of winter, the anthropogenic emissions in summer and autumn were lower. In addition, there was more precipitation during summer and autumn resulting in a moisture-based elimination, wet deposition, of atmospheric PM 10 . This elimination resulted in a lower atmospheric PM 10 concentration during summer and autumn.

PM 10 Distribution of Six Large Urban Agglomerations in China
The spatial resolution of the TOAR data provided by FY-4A was 4 km, which reflected the atmospheric PM 10 concentration distribution at the city level. Figure 8 showed the annual average atmospheric PM 10 concentration distribution of six large urban agglomerations in China. The results showed that the concentration of atmospheric PM 10 was higher in BTH (66.66 ± 16.92 µg/m 3 ), CC (64.22 ± 1 4.78 µg/m 3 ), and YRD (79.34 ± 15.86 µg/m 3 ) region. The concentration of atmospheric PM 10 in GZP and SCB was relatively low, ∼59.05 ± 14.71 µg/m 3 . The annual atmospheric concentration of PM10 in the PRD region was only 49.76 ± 6.53 µg/m 3 . According to the distribution of atmospheric PM 10 , areas of high atmospheric PM 10 concentrations in each region generally occurred in large cities and surrounding areas, which were closely related to local human activities.

Case 1: Contribution of Long-Range Transport Dust to Atmospheric PM 10 Concentration
From 14 to 17 May 2019, a large-scale dust storm occurred in northern China (35°N-45°N, 70°E-135°E). Combined with the spaceborne lidar CALIOP data, the results of the TOAR-PM 10 model were used to analyze the dust weather process. Figure 9 (Part 1) showed the three-dimensional transmission diagram of CALIOP's observational data of the dust weather process. The red transmission line was the forward trajectory line of the HYSPLIT mode. It can be observed that the dust weather originated in Taklimakan desert of China, traversed northern China to the Yellow Sea on May 17. Figure S4 in Supporting Information S1 showed the cloud and aerosol profiles obtained by CALIOP during this dust weather process. The dust aerosol ascended to an altitude greater than 8 km; consequently, it could be transmitted downstream for long distances. There was a wide range of dust aerosols at an altitude of 0-8 km in northern China, and on the 17th, there was a large area of polluted continental aerosols and polluted dust aerosols in the southern Yellow Sea. The red line in Figure 10 was the orbit of CALIOP, and the left column was the FY-4A true color map. There were many white clouds in the map, which resulted in the vacancy value of the estimated atmospheric PM 10 concentration. It can also be seen from the figure that there was a large quantities of dust  Figure S5 in Supporting Information S1 showed the 10 m wind field during dust weather, and PM 10 was the estimated value of the TOAR-PM 10 model. The wind speed in northern China was significantly greater than that in southern China. The surface wind in northern China was generally westerly. The area with high surface wind speed corresponded to the high atmospheric PM 10 concentration and dust transmission path.
As shown in Figure 9 (Part 2), it was the atmospheric PM 10 concentration (Figure 9a, Dust period) during the dust weather process (14-17 May 2019) and the atmospheric PM 10 concentration (Figure 9b, None_Dust period) without dust weather in May 2019. In addition, the difference (Figure 9c, Dust period-None_Dust period) between the two periods was presented. The left column was the station observation value, and the right column was the estimated value of TOAR-PM 10 model, and through the difference (Figure 9c)

Case 2: Changes in PM 10 Concentration Under the Combined Conditions of Dust and Haze Weather
On 24-30 November 2018, there was a large area of haze in China. In addition, there was an LRTD weather process in northern China on November 25-27 (the largest area of dust on November 26). This event was a composite pollution weather event of dust and haze weather. The haze period was November 24-30 (haze period), the dust weather period was November 25-27 (dust period), and the period of no dust nor haze weather was November 1-23 (None_Haze_Dust period). As shown in Figure 11 (Part 1), CALIOP observed the three-dimensional transmission of the dust weather process. The source and transmission path of the dust weather were similar to the dust weather process in May 2019 (as shown in Figure 9, Part 1), but the dust intensity and transmission height were less.
In Figure S6 in Supporting Information S1, a large area of dust aerosols and pollution dust aerosols were found at an altitude of 0-4 km in China from the 24th to 27th, and a small amount of dust aerosol was found at an altitude of 8 km on the 26th, which also showed that the dust intensity was less. The FY-4A true color (RGB) map in Figure 12 showed clouds (white), which was consistent with the observation of CALIOP ( Figure S6 in Supporting Information S1). From 24 to 27 November 2018, the estimated atmospheric PM 10 concentrations in China were 81.98,95.23,198.47,and 142.84 μg/m 3 (northern China: 101.32,107.38,292.72,and 207.59 μg/m 3 ), and the observed atmospheric PM 10 concentrations were 99.32,130.18,174.98,and 171.59 μg/m 3 (northern China: 122.50,193.56,302.76,and 276.10 μg/m 3 ). The difference between the estimated and observed values was due to the missing values of the estimated PM 10 caused by cloud cover. Figure S7 in Supporting Information S1 showed the wind field of the dust-weather process. The wind speed was low in the southern region and high in the northern region of China. The wind speed was greatest on November 26, which was also consistent with the   . There were two principal reasons why the estimated value of the model was less than the observed value of the station. A reason for this was the lack of data in some areas due to the existence of clouds. Second, the sample size of the model average was much larger than the number of stations on the station average. Figure 11d showed the difference in atmospheric PM 10 concentration between the haze period and the None_ Haze_Dust period. Based on the model PM 10 , during the haze period, the PM 10 in 74% of China increased by 20%, 53% of China increased by 50%, 43% of China increased by 70%, 17% of China increased by 100%, and 10% of China increased by 200%. The observed atmospheric PM 10 concentration increased by 20% at 1,327 stations (accounting for 83% of the total number of stations). That of 1,109 stations (69%) increased by 50%, that of 948 stations (59%) increased by 70%, that of 713 stations (44%) increased by 100%, and that of 204 stations (13%) increased by 200%. Figure 11e showed the results of the atmospheric PM 10 concentration comparison between the dust and haze periods, which one may estimate the contribution of LRTD to haze weather. Based on the model results, due to the LRTD transport of dust, atmospheric PM 10 concentration increased by 20% in 33% and 50% in 11% of China. Based on surface station data, atmospheric PM 10 concentration observations at 352 stations (22% of the total number of stations) increased by 20%, and that at 116 stations (7%) increased by 50%. As shown in Figure 11e, the dust weather mainly affected the PM 10 concentration in the dust transmission path areas, such as China's Hexi Corridor and Inner Mongolia.

Conclusions
The hourly atmospheric PM 10 concentrations in China were obtained using an interpretable deep learning model (DF model) and FY-4A TOAR data from June 2018 to May 2019. The main conclusions were as follows: The optimal hourly R 2 of 10-fold cross validation of TOAR-PM 10 DF model can reach 0.85 (13:00 Beijing time); The R 2 (RMSE) of daily, monthly, seasonal, and annual average were 0. In spring, the PM 10 concentration in northern China was higher than that in southern China, which may be related to the LRTD (Tao et al., 2021;L. Zhao et al., 2020). Excluding the dust weather periods, the areas with high PM 10 values in China were mainly in large cities and suburban areas, which were related to local human activities (Tao et al., 2014).
The DF model can obtain the importance of the model features. The results of the FY-4A TOAR-PM 10 model showed that TOAR, BLH, RH, surface wind speed (U10 and V10), TM, and TIME contributed significantly to the model. The performance of the model was related to the contributions of these important features (Chen, Song, Shi, & Li, 2022). The performance of the model would be worse in areas with a large contribution to surface pressure (SP). As shown in Table 3, the performance of the FY-4A TOAR-PM 10 model was better than that of other researchers using the AOD-PM 10 model. Using the same FY-4A TOAR and other auxiliary data, the DF model performed better than other traditional machine learning models (such as DT, RF, and ET).
China's arid and semi-arid regions account for ∼57% of the country's land (Y. Yang et al., 2019  The results were similar to those of others (Chen, Song, Shi, & Li, 2022;Gobbi et al., 2013;Guan et al., 2019;Remoundaki et al., 2013). The source (originating from the Taklimakan Desert in China) and transmission path of the two dust weather processes were similar, and the contribution to atmospheric PM 10 concentration in China and northern China was the same, but the intensity of the second dust weather was weaker than that of the first dust weather. In other words, the contribution of LRTD to local PM 10 was not only related to the intensity of dust weather, but also to meteorological conditions such as ground wind speed (Dimitriou & Kassomenos, 2018;Gobbi et al., 2019). In the first dust weather, the ground wind speed was large, which was conducive to the diffusion of ground pollutants and the reduction of atmospheric PM 10 concentration; The second, the low wind speed was conducive to the dry settlement of dust and the increase of PM 10 concentration. The results showed that the contribution of LRTD and local pollution to PM 10 in haze days was both important.

Data Availability Statement
The PM 10 data were obtained from the China Environmental Monitoring Center, http://www.cnemc.cn (CEMC, 2022