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Research Article
Efficient Measurement of Orbital Angular Momentum Entanglement Using Convolutional Neural Network
- Version of Record online: 17 January 2025
An efficient tomography framework for high-dimensional orbital angular momentum (OAM) entanglement is proposed, using convolutional neural networks. This method requires only two measurements to rapidly reconstruct the density matrix, even for mixed entangled states and incomplete tomographic scenarios. This approach demonstrates high fidelity and fast data processing, significantly enhancing the measurement efficiency for high-dimensional OAM entangled states.
High-Speed and Broadband n-Si/p-Se0.3Te0.7/ITO Heterojunction Photodetector
- Version of Record online: 17 January 2025
This study incorporates internal photoemission and holes trapping mechanisms to enhance the performance of Si/Se0.3Te0.7 heterojunction photodetectors, focusing on sensitivity and speed. The photodetector shows a 10000% improved responsivity at 1310 and 1550 nm, and a response time of ≈20 µs over a wide spectral range which represents a 100-fold reduction compared to devices lacking these mechanisms.
Spatially Asymmetric Optical Propagation and All-Optical Switching Based on Spatial Self-Phase Modulation of Semimetal MoP Microparticles
- Version of Record online: 17 January 2025
The SSPM ring formation dynamics of MoP microparticles are investigated, their nonlinear refractive index and ring formation time are characterized, and the formation mechanism of self-diffraction rings is analyzed. Additionally, by utilizing the superior nonlinear optical response of MoP microparticles, the spatially asymmetric optical propagation of MoP/violet phosphorus (VP) cascaded samples and the all-optical switching performance of MoP microparticles are demonstrated, respectively.
Counterintuitive Reversal of Circular Dichroism via Controllable Plasmonic Guided Mode Resonance in Diatomic Metasurfaces
- Version of Record online: 17 January 2025
The continuous variation and counterintuitive sign reversal of circular dichroism are achieved by manipulating the collective interference of plasmonic guided mode resonances within diatomic metasurfaces, providing a straightforward approach for manipulating circular dichroism without modifying the geometric chirality. Experimental demonstration showcases its potential applications in chiral optical encryption.
Synthesis and Irreversible Pressure-Induced Emission Enhancement of Ultrathin Lead-Free 2D Organic–Inorganic Hybrid Perovskite (i-OA)3BiBr6 Nanosheets at Room Temperature
- Version of Record online: 15 January 2025
Irreversible enhancement of self-trapped exciton emission in ultrathin 2D lead-free hybrid perovskite nanosheets under ambient conditions is successfully achieved. Concurrently, strengthened hydrogen bonds stabilize the crystal structure, maintaining optimal lattice distortion and ensuring the durability of the high-efficiency emission.
Second Harmonic Generation with 48% Conversion Efficiency from Cavity Polygon Modes in a Monocrystalline Lithium Niobate Microdisk Resonator
- Version of Record online: 15 January 2025
An ultra-efficiency second harmonic generation (SHG) mechanism is demonstrated by exciting ultra-high Q cavity square modes in an X-cut thin-film lithium niobate microdisk resonator without fine microdomain structures to maximum leverage the largest nonlinear coefficient d33 and the high modal overlap factor, leading to highly efficient SHG with an absolute conversion efficiency as high as 48.08%.
Photonic Terahertz Chaos Enabling High-Precision and Unambiguous Ranging
- Version of Record online: 15 January 2025
A broadband photonics-based chaos source operating at the terahertz (THz) band is generated and experimentally achieves high-precision ranging with anti-ambiguity. Facilitated by the mutual enhancement between THz radar and chaos source, this work bridges the THz gap in the practical deployment of chaos theory and will pave the way for a new regime of THz radar empowered by chaos.
Polarization-Locked Floquet Higher-Order Topological Insulators in Synthetic Dimension
- Version of Record online: 15 January 2025
A strategy based on photonic polarization inter-band transition is proposed to realize Floquet higher-order topological insulators in synthetic dimension, and the polarization-locked topological corner states are theoretically demonstrated. The proposed method manifests great flexibility in manipulating topological phase transitions. This strategy thus deepens the understanding of higher-order topology and bulk-boundary correspondence.
Pathway Selectivity in 2D Electronic-Vibrational Spectroscopy with Quantum Light
- Version of Record online: 15 January 2025
2D spectroscopy has been used for decades to study light-harvesting materials. Interpreting 2D spectra is usually challenging since multiple light-matter interaction pathways contribute to a recorded signal. This theoretical study shows how entangled photons can help record distinct 2D spectra for different pathways. Quantum entanglement between photons is shown to improve the visibility of different features in a spectrum.
Fast-Tuning and Narrow-Linewidth Hybrid Laser for FMCW Ranging
- Version of Record online: 15 January 2025
In this study, a hybrid-integrated laser source by self-injection locking (SIL) a DFB laser diode to a low-loss micro-ring resonator is presented. Benefiting from these components, a linewidth of 9 kHz, a modulation efficiency of 7 GHz/V, and a frequency excursion of 1.05 GHz in the integrated device are simultaneously achieved. Finally, we produce a linear FMCW signal with a chirp nonlinearity of 4.3 × , delivering a 0.4 cm ranging precision in this experiment is produced.
Experimental Emulator of Pulse Dynamics in Fractional Nonlinear Schrödinger Equation
- Version of Record online: 14 January 2025
The authors present an experimental emulator to investigate pulse dynamics within the framework of the fractional nonlinear Schrödinger equation. By tailoring fractional group-velocity dispersion and Kerr nonlinearity in an optical cavity, distinctive spectral-temporal phenomena, including fractional solitons and spectral valleys, are unveiled. This work deepens the understanding of fractional nonlinear systems and paves the way for exploring fractional quantum mechanics.
Ferrofluid-Assisted Dynamic Metasurface 3D Holography Endowed With Rapid, Linear, and High-Contrast Color Modulation
- Version of Record online: 14 January 2025
In this study, the results of a new ferrofluid-assisted dynamic metasurface is reported for achieving 3D holography endowed with rapid, linear, and high-contrast color modulation at the same time. This opens the door to a novel implementation of the dynamic metasurface 3D holography, transcending the currently limited display capability of metasurface holography.
Self-Induced Radioluminescence in Supramolecular Metal Halide Doped with Radioactive Isotope Strontium-90
- Version of Record online: 14 January 2025
Mechanoluminescence from Lead-Free Perovskites Cs2HfCl6: Te4+
- Version of Record online: 14 January 2025
Advanced Physical Layer Metasurface-Empowered Cryptography with Robustness, High Capacity, and Enhanced Security
- Version of Record online: 13 January 2025
A robust, high-capacity encryption method based on a dual-band complex-amplitude metasurface is proposed. By integrating ASCII encoding, a SHA-256 compressed digital signature, a multivariate encryption key, and a modified VSS scheme, security is significantly enhanced, eliminating the need for codebook transmission. Additionally, a 3D wavefront reconstruction algorithm is used to improve capacity. A metasurface sample is fabricated, and characterized as a proof-of-concept demonstration.
Hybrid Femtosecond Laser 3D Processing Technology for Rapid Integration of Functional Optical Devices on Fibers
- Version of Record online: 11 January 2025
This work proposes a hybrid femtosecond laser 3D processing system for rapid integration of 3D micro–nanostructures on fibers. This technology combines femtosecond projection lithography with direct laser writing; thus, improving efficiency by up to two orders of magnitude compared to the traditional point by point scanning strategy. No optical components need to be changed when switching processing modes.
Polarization-Independent Dispersive Complex-Amplitude Modulation via Anisotropic Metasurfaces
- Version of Record online: 11 January 2025
As well known, polarization-independent characteristic is highly desirable for practical applications, and for metasurfaces, it is typically achieved through isotropic structures. Here, counterintuitively, polarization-independent dispersive complex-amplitude modulation is achieved via a single-layered anisotropic metasurface. By fully exploiting the degrees of freedom (DoFs) in the parameter space, the previously unattainable polarization-independent functionalities can be achieved without adding additional challenges to metasurface manufacturing.
Pressure-Tailored π–π Stacking in Dimers Enhances Blue Photoluminescence in Boron-Based Organic Molecules
- Version of Record online: 11 January 2025
Pressure-treated phenylboric acid (PBA) exhibits a brilliant blue emission with a photoluminescence quantum yield from the initial 2.3 % increasing to 31.5 %. Pressure-induced phase transition enhanced hydrogen bonds, which restrict the vibration of the benzene ring and minimize the non-radiative loss. The increased probability of electronic transition and oscillator strength results in the brighter blue PL emission of PBA.
Thermal Management in AlGaAs-On-Insulator Microresonators: Enabling and Extending Soliton Comb Generation
- Version of Record online: 11 January 2025
This work demonstrates thermal management in AlGaAs-on-insulator microresonators using an auxiliary laser, enabling room-temperature soliton comb generation. By harnessing the residual thermal effects, the soliton existence range is extended to 37 GHz without active feedback. This approach paves the way for practical deployment of AlGaAs frequency comb sources, unlocking new possibilities for integrated photonics applications.
Non-Invasive Anatomical Level Cerebrovascular Imaging of Mice Using Diffusion Model-Enhanced Fluorescence Imaging
- Version of Record online: 10 January 2025
In vivo indocyanine green (ICG) -based fluorescence imaging is promising for cerebrovascular visualization but faces limitations due to skull interference, often requiring invasive methods. The diffusion models non-invasively enhance trans-scalp images to an anatomical level resolution similar to trans-cranial images (20.1 µm). Tested on a stroke model, it offers a cost-effective, high-resolution alternative for detecting ischemic sites.
Speckle-Free 3D Holography in the Wigner Domain
- Version of Record online: 10 January 2025
In this work, an ideal numerical light field mapping physical model from the hologram plane to the 3D image plane is established with the aid of the Wigner distribution function, which allows the analysis of a light field from the space and the spatial frequency domains simultaneously. Furthermore, by introducing a comprehensive optimization into hologram encoding, speckle-free 3D holography in the Wigner domain is achieved.
Room-Temperature and Ultrafast Synthesis of Sub-4 nm Yb3+/Nd3+ Ions-Doped CaMoO4 Nanocrystals with Near-Infrared Photoluminescence Quantum Yield of 40%
- Version of Record online: 10 January 2025
Dynamic Multicolor Display with Wide Color Gamut Enabled by Vanadium Oxide-Based Fabry–Pérot Electrochromic Nanocavities
- Version of Record online: 10 January 2025
A wide color gamut electrochromic display utilizing asymmetric VOx-based Fabry–Pérot nanocavities is presented. This design enables exceptional color modulation from a single electrode, achieving dynamic transitions across magenta, purple, blue, and green hues by adjusting the VOx film thickness. Structural analysis reveals the role of Li+ ions dynamics in influencing optical properties, facilitating advanced applications in flexible display electronics.
Significant Non-Reciprocal Transmission Achieved by Combining Nonlinear Near-Zero Index Materials with Bound States in the Continuum
- Version of Record online: 09 January 2025
A zero-index BIC is realized in an asymmetric nonlinear silicon metasurface. Because of the high Q-factor of quasi-BIC and the enhanced nonlinear effect in the near-zero index background, a large range of non-reciprocal transmission of ≈7.1 at low pump intensity is realized. For the first time, quasi-BIC with ZIM are combined together to enhance nonlinear effects, which may be of great significance for the application involving nonlinear effects.
MASCN Vapor-Assisted Fabrication of Compact and Large-Grain MAPbI3 Polycrystalline Wafer for X-Ray Detection and Imaging
- Version of Record online: 09 January 2025
This study demonstrates a thiocyanate salt vapor-assisted hot-pressing method for fabricating MAPbI3 polycrystalline wafer X-ray detectors. During hot pressing, MASCN vapor facilities in situ growth of MAPbI3 crystal grains, leading to remarkable X-ray detection performance, including a high sensitivity of 16611 µC Gyair−1 cm−2, a low detection limit of 47.5 nGyair s−1, robust operational stability, and superior imaging capability.
Chiral-Gain Photonics
- Version of Record online: 09 January 2025
This work explores potential applications of chiral-gain materials, whose electromagnetic response can be active or dissipative depending on the wave spin angular momentum. It is shown that these materials enable unique devices, including chiral lasers, polarization-dependent mirrors, and coherent-perfect-absorber lasers, while also bypassing reciprocity constraints to enhance coupling in high-Q cavities.
Multi-Watt Long-Wavelength Infrared Femtosecond Lasers and Resonant Enamel Ablation
- Version of Record online: 09 January 2025
A 6–12 µm broadband tunable femtosecond parametric amplifier, generating output power of 2.4 W at 7.5 µm, and 1.5 W at 9.5 µm is presented. Efficient resonant ablation and microstructure fabrication on enamel at the hydroxyapatite resonant wavelength of 9.5 µm is also showcased, with a laser intensity two orders-of-magnitude lower than that required by non-resonant counterparts.
Efficient Emission of Lanthanide Ion in Double Perovskite Nanocrystals Enabled by Synergistic Effect of Energy Level Modulation and Crystal-Field Engineering
- Version of Record online: 08 January 2025
The localized distortion of the crystal field induced by K+ ions doping causes energy level splitting of Sb3+ ions, resulting in more effective energy transfer efficiency from the host to Ln3+ ions, simultaneously introducing opposite odd parity, and breaking the forbidden transition rule, promoting luminescence intensity of Ln3+ ions.
NIR-to-NIR Lifetime Based Thermometry with the Thermally Elongated Luminescence Kinetics Driven by Structural Phase Transition in LiYO2:Yb3+
- Version of Record online: 08 January 2025
In this work, an approach is presented that utilizes a thermally induced increase in the symmetry of the host material associated with a structural phase transition in LiYO2:Yb3+ enabling modification of the probability of radiative depopulation of the 2F5/2 state of the Yb3+ ion and shape of the emission spectra for luminescence thermometry.
3D Terahertz Confocal Imaging with Chromatic Metasurface
- Version of Record online: 07 January 2025
A passive terahertz focusing metasurface is designed to achieve frequency-dependent focal lengths while maintaining a constant spot size. It enables 3D see-through non-metallic objects with fixed spatial resolution across a large depth-of-field. The proposed metasurface can be employed in various applications, including in-situ defect detection, object inspection in security screening, and hidden layer identification in cultural heritage preservation.
Chirp-Managed, High-Energy, Low-Repetition Mamyshev Oscillator Based on Hollow Core Fiber
- Version of Record online: 06 January 2025
This paper demonstrates a new method of combining Hollow-core fiber (HCF) and Mamyshev oscillator techniques to generate high-energy ultrashort pulses at a low-repetition. In addition to lowering the pulse frequency, the HCF provides chirp-managed functionality in the Mamyshev oscillator, which further enhances the maximum achievable pulse energy. A high-energy (514 nJ), short-pulse (46 fs), and low-repetition (1 MHz) fiber laser is successfully realized.
Tailored Metal-Oxygen Bonding in Amorphous Perovskite CoSnO3 for Broadband Ultrafast Laser State Active Manipulation
- Version of Record online: 06 January 2025
In this study, an ion-exchange strategy is utilized to effectively tailor the metal-oxygen bonds in amorphous CoSnO3, resulting in Fe-doped CoSnO3 (Fe-CoSnO3). Experimental results demonstrated that the toleration of metal-oxygen bonds in CoSnO3 accelerated the electron transition rate, shortened the recovery time, and significantly enhanced its nonlinear optical (NLO) properties, actively manipulating the mode-locking laser state in the NIR region.
Abnormal Unidirectional Lasing from the Combined Effect of non-Hermitian Modulated Bound States in the Continuum and Fabry–Pérot Resonance
- Version of Record online: 06 January 2025
A parity-time (PT) symmetry grating results in an asymmetric split of bound states in the continuum (BIC). Based on the joint effect of the asymmetric PT-BICs and cavity resonance, a line source produces unidirectional and single mode lasing with an interesting wavefront transformation: from a diverging wave to a unidirectional plane wave.
Adaptive Structured-Light 3D Surface Imaging with Cross-Domain Learning
- Version of Record online: 06 January 2025
A cross-domain learning framework for adaptive structured-light 3D imaging is proposed, enhancing generalization across diverse systems and environments. The method incorporates a novel mixture-of-experts architecture, significantly improving performance over traditional specialist and generalist DNNs, and advancing robust AI-driven optical metrology.
KTb3−xGdxF10 Nano-Glass Composite Scintillator with Excellent Thermal Stability and Record X-Ray Imaging Resolution
- Version of Record online: 04 January 2025
Scintillators exhibiting both excellent spatial resolution and thermal stability are highly sought after for X-ray imaging and radionuclear detection applications in harsh environments. By employing a suite of techniques—including phase-separation-assisted crystallization, energy transfer, and compensation—Tb3+-doped nano-glass composite (nano-GC) scintillators are developed with good scintillation performance, rendering it particularly suited for high-temperature X-ray imaging applications.
Anisotropic Third-Harmonic Vortex Beam Generation with Ultrathin Germanium Arsenide Fork Gratings
- Version of Record online: 03 January 2025
Highly anisotropic third-harmonic (TH) optical vortex beam generation is demonstrated with fork grating holograms patterned on ultrathin 2D GeAs flakes. The TH optical vortices with defined topological charges are produced and strong anisotropy ratios of TH vortices are observed. These results pave the way toward the advancement of 2D material-based anisotropic nonlinear optical devices.
Achieving over 500% Improvement in Optical Efficiency for VHOE-Lightguide Near-Eye Glasses with Exit Pupil Expansion
- Version of Record online: 03 January 2025
This paper proposes an optimized spectrum distribution of the input image to significantly enhance the optical efficiency of volume holographic optical element (VHOE)-based lightguides with exit pupil expansion (EPE). The concept is proved by applying a dispersion holographic optical element. It yields an optical efficiency of 9% for the lightguide with a 30° field of view, representing a 5.63-fold improvement over conventional VHOE-based EPE lightguides.
A Universal Strategy for Multicolor Mechanoluminescence via Radiative Energy Transfer Based on Ultraviolet Mechanoluminescent Material Ca9Al(PO4)7:Ce3+
- Version of Record online: 03 January 2025
This work introduces a universal strategy for achieving multicolor mechanoluminescence (ML) through radiation energy transfer by ultraviolet ML material. Using this strategy, certain highly efficient photoluminescence materials can develop ML, transitioning from nonexistent to present or from weak to strong. Additionally, the ML color can be tuned by adjusting the composition ratio of energy donor and acceptor.
Highly Efficient Acousto-Optic Modulation Driven by Ultra-Low Power in Integrated Photonic–Phononic Waveguides
- Version of Record online: 02 January 2025
Achieving efficient acousto-optic modulation remains challenging due to the simultaneous requirements of confinement and minimal loss for acoustic and optical fields. Using integrated gallium nitride waveguides, these limitations are addressed and complete mode conversion with a 1.67-mW driving power, setting a benchmark for integrated acousto-optics, is demonstrated. That enables new possibilities for integrated quantum and classical signal processing.
Observation of Lossless Topological Bound States from Non-Hermitian Subspaces
- Version of Record online: 02 January 2025
A three-layer Su-Schrieffer-Heeger (SSH) chain is designed and demonstrated via femtosecond laser direct writing. The system can be split into a Hermitian SSH subspace and a non-Hermitian ladder subspace through hidden symmetry, resulting in the observation of lossless topological bound states in a non-Hermitian system. Such a system offers the potential for achieving coherent topological propagation on photonic chips.
Unlocking Secure Optical Multiplexing with Spatially Incoherent Light
- Version of Record online: 02 January 2025
While coherent light shows great potential for optical multiplexing, its susceptibility to environmental disturbances often results in information loss. Hereto, an incoherent optical information multiplexing protocol leveraging the field correlations of structured random light is proposed. The inherently incoherent nature of random light makes this protocol have high security, high capacity, and high fidelity, even in an extremely noisy environment.
Highly Emissive Organic Cuprous Halides with [Cu4Br6]2− Unit for X-Ray Imaging
- Version of Record online: 02 January 2025
Three organic-inorganic hybrid cuprous halides with [Cu4Br6]2- unit, namely (TMAA)2Cu4Br6, (EtTPPh)2Cu4Br6, and (MtTBA)2Cu4Br6, are designed and synthesized. (TMAA)2Cu4Br6 exhibits a near-unity PLQY up to 99.86%, which can be attributed to the suppression of non-radiative transition by the introduction of rigid cations. The scintillation film fabricated by (TMAA)2Cu4Br6 achieves a spatial resolution of up to 15.6 lp mm−1. This work presents a promising strategy for designing hybrid cuprous halide scintillators.
Pressure-Synergistic Ligand Engineering Toward Enhanced Emission and Remarkable Piezochromism in Cadmium Sulfide Nanocrystals
- Version of Record online: 02 January 2025
A robust strategy is developed through pressure-synergistic ligand engineering to achieve enhanced emission and remarkable piezochromism from orange to blue-violet emission with high color purity of 71.4% in the synthesized cadmium sulfide nanocrystals that exhibits both band-edge emission and strong defect emission.
Dual Jones Matrices Empowered Six Phase Channels Modulation with Single-Layer Monoatomic Metasurfaces
- Version of Record online: 01 January 2025
This work proposes a dual Jones matrices operation in both linear and circular polarization bases to extend the independent manipulation of the Jones matrix phase channels to a counter-intuitive and unprecedented number of six using a single-layer monoatomic metasurface. A modified three-step gradient descent algorithm is introduced to encode six holographic images, opening new avenues for optical wavefront manipulation.
Microwave-Optics Entanglement via Coupled Opto- and Magnomechanical Microspheres
- Version of Record online: 31 December 2024
A new mechanism to generate microwave-optics entanglement is proposed using two coupled opto- and magnomechanical microspheres (a silica sphere and an yttrium-iron-garnet sphere) placed inside a microwave cavity. This is realized by activating the magnomechanical parametric down-conversion yielding the magnomechanical entanglement, which is eventually distributed to the microwave and optical cavities through the magnon-microwave, mechanics-mechanics, and optomechanical beamsplitter interactions.
High-Performance Chiral Mode Switching Devices Using Silicon Metamaterial Waveguides Beyond 1.55 µm
- Version of Record online: 30 December 2024
This study uses metamaterial waveguides to overcome wavelength-dependent mode mismatches, enabling ultra-broadband, high-purity chiral mode switching beyond 1.55 µm. Simulations spanning both the optical communication and 2 µm wavebands show near-unity transmission efficiency and high mode purity (> 98.8%) across a record 500 nm bandwidth. The work advances high-efficiency, high-purity chiral transmission devices in the near/mid-infrared, with promising prospects for EP-based applications.
Resonant Meta-Lens in the Visible
- Version of Record online: 30 December 2024
An all-dielectric resonant meta-lens based on the Fresnel zone plate design is developed to enable wavelength-selective focusing. It achieves reflective focusing at a resonant wavelength of 460 nm while allowing normal transmission at non-resonant wavelengths. Simulation (experimental) results indicate a high color purity of 90% (66%). Additionally, a multi-resonant meta-lens has been proposed to focus selectively on three colors.
Review
Recent Advances in Plasmonic Sensing Techniques for Exosome Detection and Composition Analysis
- Version of Record online: 30 December 2024
A comprehensive summary of various plasmonic sensing techniques, focusing on both propagating SPR (PSPR) and localized SPR (LSPR) platforms is presented. Their characteristics, sensing performances, and practical applications in exosome capture and detection are demonstrated, including current challenges and future research directions in this field, offering insights into the potential of plasmonic sensing in biomedical research and clinical practice.
Research Article
Integrated Photonic Nonreciprocal Devices Based on Susceptibility-Programmable Medium
- Version of Record online: 30 December 2024
An optical medium is proposed with programmable susceptibility tensor based on polarizable atoms, enabling efficient control of the optical response in space and time. It highlights the potential for nonreciprocal optical effects and rapid, reconfigurable signal isolation in atom-cladded waveguides, offering significant advancements for integrated photonic devices and structured optics.
Review
Integrated Optical Spectrometers on Silicon Photonics Platforms
- Version of Record online: 27 December 2024
In this review article, diverse strategies are employed to enhance the performance of integrated optical spectrometers on silicon photonics platforms, revealing the underlying principles, diverse design methodologies, and spectral performances inherent in distinct device architectures. Building upon these insights, this review goes a step further to navigate the challenges these innovations face and the potential applications they unlock.
Research Article
Ultra-Low-Loss and Athermalized Lithium-Niobate-on-Insulator Photonic Chip for Next-Generation PONs
- Version of Record online: 27 December 2024
A high-capacity lithium-niobate-on-insulator (LNOI) optical transmitter for next-generation passive optical-networks (PONs) is proposed and demonstrated with ultra-low temperature-dependence for the first time by simultaneously introducing Z- and Y-propagation LNOI photonic waveguides. Here, the corresponding photonic filters are realized by integrating amplitude-apodized multimode waveguide gratings (MWGs) and mode (de)multiplexers designed with Z-propagation LNOI photonic waveguides, which are found to be with a low thermo-optic coefficient and thus enable the athermalization. Meanwhile, the high-speed optical modulators connected at the add ports of the photonic filters for the 1342/1577 nm channels are developed with Y-propagation LNOI photonic waveguides with the maximal electro-optic effect. For the fabricated on-chip optical transmitter, box-like spectral responses are achieved with ultra-low excess losses of < 0.5 dB and low inter-channel crosstalk of < −26 dB for all the channels whose bandwidths are respectively ∼16/20/4/15/5 nm as expected. The present LNOI photonic chip is nearly athermal in experiments, exhibiting very low temperature-dependence less than 8.7 pm °C−1 in the full wavelength range of >300 nm. Finally, high-capacity data transmissions of 50/100 Gbps on-off keying (OOK) signals and 100/200 Gbps PAM4 signals are demonstrated, providing a promising solution for next-generation PONs.
Variational Learning of Integrated Quantum Photonic Circuits via Genetic Algorithm
- Version of Record online: 27 December 2024
This work presents a variational learning approach that integrates post-selection and fundamental photonic components to enable real-time optimization of chips tailored to specific tasks and simplifying complex circuits into single nonlinear operators. The design of a single ancilla CNOT gate and the first demonstration of quantum stochastic simulation using integrated photonics is achieved, showing great promise for quantum information processing.
Remarkable Energy Transfer Efficiency in Spatially Separated 2D Heterostructure via Establishing Entangled States by Bloch-Surface Plasmon Polariton
- Version of Record online: 27 December 2024
In the designed Ag nanoholes/WS2/SiO2/MoS2 heterostructures, A exciton of WS2 and spatially separated B exciton of MoS2 are entangled by the Bloch-surface plasmon polariton mode. Such entangled states assist in remarkably efficient energy transfer. This research can establish the scientific foundation for developing the related heterostructure optoelectronic devices.
Micro-Rotors on Frictional Solid Surfaces via Optothermally-Invoked Chirality
- Version of Record online: 27 December 2024
The article demonstrates the realization of microscopic rotors adhered on frictional solid surfaces using an all-optical approach. Through an opto-thermo-elastic coupled mechanism, a pulsed laser reshaped to possess an elongated Gaussian field injects chirality in optothermally excited elastic waves within the obliquely irradiated rotor, which in turn induces a frictional torque empowering the rotational motion of the rotor.
Far-Field and Near-Field Manipulation via Multipole Coupling Phenomenon in Van der Waals Metasurfaces
- Version of Record online: 26 December 2024
Metasurfaces fabricated from van der Waals material make it possible to excite octupole quasi-trapped modes without violating the symmetry properties of the system and to observe narrowband features in light reflection spectrum for the metasurface accompanied by the strong localization of near-field energy in its plane.
High-Resolution Non-Line-of-Sight Tracking By Comb-Calibrated FMCW LiDAR
- Version of Record online: 26 December 2024
A real-time comb-calibrated FMCW LiDAR system is demonstrated for high-resolution NLOS tracking. A 3D positioning (and velocity) accuracy of 2 mm (and 2 mm s−1) and the capability to realize real-time multi-object tracking are demonstrated in experiment. Importantly, the FMCW-LiDAR approach can obtain the position and velocity of multiple objects in a snapshot, thus resolving the problems of measurement origin uncertainty, false alarm, and detection overlap.
All-Dielectric Meta-Microlens-Array Confocal Fluorescence Microscopy
- Version of Record online: 24 December 2024
A meta-microlens array (meta-MLA) confocal microscope is presented that enhances fluorescence imaging speed without replacing existing scanning devices. The use of ultra-compact metasurface enables rapid image acquisition and reduces photo-bleaching. Image clarity comparable to traditional systems is maintained by integrating deep learning and deconvolution methods. The approach is versatile and compatible with current biomedical imaging applications.
Multifunctional Metalens for Trapping and Characterizing Single Atoms
- Version of Record online: 24 December 2024
A multifunctional metalens that integrates an achromatic lens with large numerical aperture is demonstrated, a quarter-wave plate, and a polarizer for trapping and characterizing single Rubidium atoms. The metalens can simultaneously focus a trapping beam at 852 nm and collect single-photon fluorescence at 780 nm.
Unconventional Photo-Control of Structural Features Using Elliptically Polarized Light
- Version of Record online: 24 December 2024
An ellipticity-controlled spatially multiplexed surface modulation is demonstrated using orthogonal elliptically polarized beams. This technique enables slightly distorted unique structural features, offering enhanced spatial control over azopolymer migration and consequently diffracted light. This advancement enables the fabrication of complex structures like Fourier Optical Elements and Photonic Crystals.
3D Orbital Angular Momentum Multiplexing Holography with Metasurfaces: Encryption and Dynamic Display of 3D Multi-Targets
- Version of Record online: 23 December 2024
So far, multiplexing holographic technology of 3D multi-targets is still a blank. Here, the conception of 3D orbital angular momentum (OAM) multiplexing holography is proposed. Holographic encryption and dynamic display for 3D multi-targets are realized experimentally for the first time with metasurface. This breaks the restriction that only 2D images can be encrypted in traditional holographic encryption.
A Strong Red-Emitting Phosphor-in-BASK-Glass through Spark Plasma Sintering: Insights into the Role of Interfacial Reaction on PL Efficiencies
- Version of Record online: 23 December 2024
Red-emitting phosphor-in-glass (Red-PiG) color converters are essential for high-power light-emitting diode and laser lighting applications, but face challenges due to degradation and interfacial reactions. This study demonstrates how spark plasma sintering effectively mitigates these issues, optimizing interfacial morphology to achieve a borosilicate-based PiG with a luminous flux of 248 lm and efficiency of 173 lm W−1, setting new performance benchmarks.
Dion-Jacobson Phase Mn2+-Doped Perovskite Scintillators for High-Resolution X-Ray Imaging
- Version of Record online: 23 December 2024
All-Optical Coherent Control of Ultrafast Injection Photocurrent in Multilayer Rhenium Disulfide Under Two-Color Light Excitation
- Version of Record online: 23 December 2024
The coherent ultrafast injection photocurrent by quantum interference in low-dimensional semiconductors can be veiled by other linear or nonlinear optical effects. A method is proposed to isolate the pure injection photocurrent from optical responses of multilayer rhenium disulfide (ReS2), based on the terahertz (THz) emission spectroscopy under two-color light excitation. This work promotes the ultrafast quantum coherent control for solids.
Hybrid Thin-Film Lithium Niobate Micro-Ring Acousto-Optic Modulator with Low Half-Wave-Voltage-Length Product
- Version of Record online: 23 December 2024
A hybrid thin-film lithium niobate (TFLN) micro-ring acousto-optic modulator (AOM) is demonstrated. In the experiments, the double-arm micro-ring acousto-optic modulation is confirmed in a non-suspended chalcogenide (ChG)-loaded TFLN waveguide platform. The half-wave-voltage-length product VπL of the hybrid micro-ring AOM is as small as 9 mV cm. Highly efficient micro-ring acousto-optic modulation thus provides new opportunities for expanding TFLN-ChG hybrid piezo-optomechanical devices.
QCL-Based Cryogen-Free THz Optical Wireless Communication Link
- Version of Record online: 23 December 2024
A novel QCL-based, cryogen-free, and transportable wireless communication system is presented operating at 2.83 THz. The QCL device is mounted in a compact Stirling refrigerator, while a room-temperature graphene-based FET is used as a receiver, implementing a binary on-off keying (OOK) modulation scheme with Manchester encoding. Precise communication tests are performed and propose a propagation model to extrapolate the performances of an optimized configuration.
Guided-Mode Resonance Polarization-Sensitive Narrowband InGaAs Photodetector
- Version of Record online: 23 December 2024
A polarization-sensitive narrowband InGaAs photodetector (PD) operating in the short-wave infrared range is proposed, capable of capturing wavelength, intensity, and polarization data concurrently without additional optical components. The device is formed by integrating an InGaAs PD onto a silicon grating, utilizing the guided-mode resonance effect to amplify absorption at specific target wavelengths, which is different for TE and TM polarized light.
D-Band MUTC Photodiode Module for Ultra-Wideband 160 Gbps Photonics-Assisted Fiber-THz Integrated Communication System
- Version of Record online: 23 December 2024
This article introduces a high-performance MUTC-PD module with WR-6 waveguide output for photonics-assisted fiber-THz wireless communications. With flat PD chip response, low-loss transition circuits as well as optimized packaging process, the module achieves ultra-wideband and high-speed performance, supporting data rates up to 160 Gbps with 16 QAM, showcasing its potential for next-generation, high-speed communication systems.
A New Thermodynamic Approach to Multimode Fiber Self-cleaning and Soliton Condensation
- Version of Record online: 21 December 2024
A new thermodynamic theory for optical multimode systems is presented, based on a weighted Bose–Einstein law (wBE) and including a state equation, fundamental equation for the entropy and an accuracy metric. An experimental comparison of two propagation regimes of a multimode optical fiber is carried out in terms of wBE, namely the self-cleaning in the normal chromatic dispersion region of the fiber, and the soliton condensation in the anomalous dispersion region. Surprising similarities are found in terms of thermodynamic parameters such as the optical temperature, chemical potential, Boltzmann and Shannon entropy.
Exceptional-Point-Enhanced Superior Sensing Using Asymmetric Coupled-Lossy-Resonator Based Optical Metasurface
- Version of Record online: 20 December 2024
The manuscript entitled “Exceptional-point-enhanced superior sensing using asymmetric coupled-lossy-resonator based optical metasurface” by Nag Chowdhury et al presents a novel scheme for exceptional-point based quantum-enhanced-sensing using non-Hermitian asymmetric coupled-lossy-resonators, experimentally demonstrating the detection of recombinant spike-proteins of SARS-CoV-2-Omicron-strain with 〉2200% enhancement. The work provides a new perspective in high-sensitivity disease detection and monitoring with broad implications in biomedical-instrumentation and quantum-sensing.
Fiber Tip Empowered by Axial-Asymmetric Four-Sector Nanostructure for Broad-Angle Light Coupling
- Version of Record online: 18 December 2024
Realization of a Chiral Topological Whispering-Gallery-Mode Cavity in Gyromagnetic Photonic Crystals
- Version of Record online: 18 December 2024
The work reports the first experimental realization of a tunable chiral topological whispering-gallery-mode (WGM) cavity in gyromagnetic photonic crystals with time-reversal symmetry (TRS) breaking. The study experimentally demonstrates that the chiral topological WGM cavities exhibit superior robustness, and the resonance frequencies and free spectral range (FSR) of the cavities can be tuned at will by inserting a metallic scatterer with different lengths.
Flow-Based Electromagnetic Information Recovery for Inaccessible Area and Low-Resolution Detection
- Version of Record online: 18 December 2024
Sculpting electromagnetic (EM) waves to convey information is a mainstream paradigm in EM and optics applications. A flow model is proposed to explicitly calculate the conditional distribution between partially accessible EM information and comprehensive EM information, transcending the limits of conventional paradigms. This approach enables the restoration of detected EM field under diverse occlusion scenarios, without necessitating elaborate equipment.
Photon-Efficient, Hybrid Illumination for High-Throughput Fourier Ptychographic Phase Microscopy Using Lenslet-Integrated LED Illuminator
- Version of Record online: 18 December 2024
A novel high-throughput, stitching-free FPM strategy that combines a photon-efficient, lenslet-array-integrated LED illuminator with a hybrid multiplexed illumination scheme is introduced. The illuminator provides vignette-free, high-intensity illumination, dramatically reducing DF acquisition time to a few milliseconds and eliminating vignetting-induced artifacts. Meanwhile, the illumination multiplexing scheme significantly reduces the number of measurements, achieving a 0.51-NA resolution across a field of view of 4.1 mm2.
Random Holography: Generating EPR-Like Correlation with Thermal Photons
- Version of Record online: 18 December 2024
In this study, pairwise thermal photons, generated in the proposed random holography (RH), can exhibit both Hanbury–Brown–Twiss (HBT)-type and Einstein–Podolsky–Rosen (EPR)-like correlations. The experiments have demonstrated the standard EPR inequalities for position-momentum and angular position-momentum after subtracting the intensity background. The study will refresh the understanding of photon correlation and provide a simple bi-correlation light source for diverse quantum-mimic applications.
Monolithically Integrated Ultra-Low Threshold GeSn-on-Insulator Laser Using Rapid Melting Growth
- Version of Record online: 18 December 2024
The ultra-low threshold GeSnOI laser is demonstrated using a defect-free and tensile-strained GeSn layer grown by the RMG method. Ultra-low threshold of 0.52 kW cm−2 at 10 K is achieved. The RMG method can allow obtaining truly monolithic, high-performance on-chip lasers with ideal GeSn gain media, potentially completing the missing piece of the monolithically integrated Si photonics platform.
Colorful Narrow-Band Organic Polariton Light-emitting Diodes Based on a Single Emitter
- Version of Record online: 18 December 2024
Orthogonal-Based Reconfigurable Light-Controlled Metasurface for Multichannel Amplitude-Modulation Communication
- Version of Record online: 16 December 2024
Through controlling the luminous intensity of LED array beads in horizontal and vertical directions, the photoresistor value can be adjusted. Based on this characteristic, the designed metasurface can synthesize different polarized waves under x-polarized and y-polarized waves simultaneous incidence. Meanwhile, it can also realize multi-polarization amplitude modulations for information transmission under different polarized waves incidence.
2D/Quasi-2D/3D CsPbIxBr3–x Vertical Heterostructures for High-Performance Infrared-Blind Visible-Light Photodetectors Toward Imaging Application
- Version of Record online: 16 December 2024
A facile and universal strategy to construct 2D/quasi-2D/3D CsPbIxBr3–x heterostructures is proposed through the two-step phenylethylammonium bromide sequential surface treatment. The heterostructure contributes to high-performance infrared-blind visible-light photodetectors with recorded external quantum efficiency, high linear dynamic range, and fast response speed. It stimulates high-quality visible-light detection in image sensors, biomimetic eyes, and underwater wireless light communication.
Explicit Symmetry Breaking of Generalized Angular Momentum by Second-Harmonic Generation in Underdense Plasmas
- Version of Record online: 16 December 2024
The conservation law of the generalized angular momentum (GAM) of light is investigated through second-harmonic generation in inhomogeneous plasmas. The study reveals that the symmetry and topological properties of the GAM state are broken with such a nonlinear process that relies on quadrupolar interaction. Importantly, this symmetry breaking offers a readily detectable signature of the topology of the driving field.
Transparent Composite for Cooperative Near-infrared and X-ray Imaging
- Version of Record online: 16 December 2024
The highly transparent glass composite activated with Cr3+ is fabricated via controllable nanocrystallization. It exhibits tunable photoluminescence and radioluminescence response in the NIR region, with excellent external quantum efficiency and robust thermal quenching resistance. Benefiting from these distinctive features, further the cooperative imaging system is constructed and the simultaneous visualization of bone and blood is successfully demonstrated.
The Scintillating Dynamics of Self-Trapped Exciton Endowed/Unendowed by Thermally Activated Delayed Fluorescence
- Version of Record online: 14 December 2024
Unique Spectral Broadening Induced by Exchange Coupling Between Cr3+ Ions in LiAl5O8:Cr3+ Phosphors for Versatile Optical Applications
- Version of Record online: 14 December 2024
The work presents a strategy for precise control of the exchange coupling between Cr3+ ions in LiAl5O8: Cr3+ phosphor. By combining crystal field engineering and heavy doping, the NIR emission shifts from narrowband emission of isolated Cr3+ to unusual broadband emission of Cr3+-Cr3+ aggregation, which provides new insights for NIR phosphors in NIR pc-LEDs and optical thermometry applications.
Orbital Angular Momentum of Structured Vortex Beams Induced by Intensity Singularity
- Version of Record online: 13 December 2024
An effective scheme for generating structured vortex beams and orbital angular momentum from the viewpoint of intensity singularity is developed. Such structured beams exhibit intensity gradient and phase gradient. This approach possesses the advantages of simplicity, versatility, and intuition, and allows to precisely controlling the beam trajectory, intensity, and phase distribution.
Hydrogen-Sensitive Inks with 4D Printing of a Fiber-Tip Hydrogen Microsensor
- Version of Record online: 12 December 2024
An H2-sensitive photoresist, doped with palladium nanoparticles, has been developed for laser direct writing of MEMS H2 sensors. This work demonstrates that, by preparing an ultra-compact fiber-tip clamped-beam microsensor for rapid and sensitive H2 detection. Such strategy provides a solution for achieving on-chip direct laser writing of integrated H2 microsensors.
Designing a Heteroleptic Tetrahedral Group with an Ultrahigh Polarizability Anisotropy by Optimizing the Bonding Electrons Activity and Their Distribution
- Version of Record online: 12 December 2024
The introduction of heteroanions into tetrahedral groups can induce a high polarizability anisotropy, originating from the optimization of the bonding electrons activity and their distribution. Then, an elegant hetero-two-site heteroleptic tetrahedron [SO2NH2Cl] with a high polarizability anisotropy is designed, which adequately confirms the ideas in theoretical and experimental results.
Programmable Metamaterial for In-Plane Electromagnetic Wave Control in the Microwave Range
- Version of Record online: 12 December 2024
Decoupling the Conductivity–Fluorescence Tradeoff of SnO2 Nanocrystals for Efficient and Stable Quantum Dot Light-Emitting Diodes
- Version of Record online: 11 December 2024
SnO2 nanocrystals offer a promising alternative as an electron-transporting material, potentially addressing the stability issues of quantum dot light-emitting diodes (QLEDs) caused by ZnO. This study explores the effects of low-level Sb doping in SnO2 and introduces a gradient doping strategy for decoupling the fluorescence-conductivity tradeoff, setting a new benchmark for the performance of ZnO-free QLEDs.
Wavelength Decoupling Based on Minimalist Metasurfaces Enabling Bicolor Display and Information Encryption
- Version of Record online: 11 December 2024
Minimalist metasurfaces characterized by a single-celled configuration, composed of only two types of nanobricks are propsed. The design exhibits versatility, enabling wavelength decoupling for both co-polarization and cross-polarization incidence. Additionally, by integrating the metasurface with liquid crystal devices, efficient information encryption can be achieved, demonstrating broad potential applications in optical data storage, image display, and information security.
Review
Integrated Optical Tunable Delay Line and Microwave Photonic Beamforming Chip: A Review
- Version of Record online: 10 December 2024
This paper provides an extensive review of integrated optical tunable delay lines (OTDLs) and microwave photonic (MWP) beamforming chips. It covers classification, principles, calibration, control technologies, and system verification, highlighting the challenges faced in real-world applications and outlining future development directions.
Research Article
Exciton Thermodynamics in Pure Diamond
- Version of Record online: 10 December 2024
Introducing external excitation power reveals the interrelated thermodynamic properties of exciton, electron–hole plasma, and electron–hole droplet in diamond. This work presents a novel method to study luminescent thermodynamics in indirect-bandgap semiconductors, integrating power and temperature dimensions for a deeper understanding of their luminescent behavior.
Computational Imaging Encryption with Steganography and Lanthanide Luminescent Materials
- Version of Record online: 09 December 2024
A universal computational imaging fluorescent encryption framework is achieved by combining advanced lanthanide luminescent material, improved single-pixel encryption, and digital steganography. This scheme can efficiently and flexibly achieve three-level encryption of various images and convenient image acquisition by a camera, demonstrating the highly invulnerable and flexible computational fluorescent encryption and decryption application for lanthanide luminescent material.
Deterministic Parity-Time Symmetry Single-Mode Oscillation in Filterless Multimode Resonators
- Version of Record online: 09 December 2024
Deterministic single-mode oscillation in a PT-symmetric multimode resonator is achieved through saturable absorption and one-shot injection, without the need for any filter. A PT-OEO demonstrates oscillation at desired frequencies from 1.8 to 9 GHz, with ultra-low phase noise at −158.6 dBc Hz−1@10 kHz, significantly enhancing signal quality and performance without complex frequency tuning structures.
Mid-Infrared on-Chip Soliton Self-frequency Shift in Chalcogenide Glass Waveguide
- Version of Record online: 09 December 2024
Perovskite Video Camera
- Version of Record online: 09 December 2024
Combining a high-performance perovskite photodetector with a computational imaging algorithm, a perovskite video camera has been developed that can demonstrate video imaging of moving objects at a frame rate of 25 frames per second. In addition, the 1024×1024 pixel imaging captured by the perovskite camera shows the highest pixels in previous state-of-the-art perovskite imaging reports.
Lattice-Matched BaClF/CsPbBr3 Heterostructure with Enhanced and Stable Cyan Emission to Overcome Blue Overshoot and Cyan Gap of White Light-Emitting Diodes
- Version of Record online: 09 December 2024
High brightness and ultra-stable cyan-emitting BaClF/CsPbBr3 perovskite heterostructures are successfully prepared using a lattice matching strategy, which effectively overcomes the blue overshoot and cyan gap issues in white light-emitting (WLED), thereby increasing the color rendering index (CRI) from 70.1 to 86.2 and boosting the luminous efficiency from 21.3 to 87.8 lmW−1.
Ultra-Large Bandwidth and Ultra-High Sensitivity Germanium/Silicon Avalanche Photodiode
- Version of Record online: 09 December 2024
This work demonstrates a germanium/silicon avalanche photodiode (APD) with a record-large bandwidth of 67 GHz, enabling data reception of 240 Gb s−1 signal—the highest single-channel bitrate among all reported APDs. This breakthrough is achieved by implementing an extremely narrow multiplication layer to enhance the space charge effect. This work paves the way for high-speed and high-sensitivity optical interconnection.
Disentangling Structural Domains in Solution-Processed 2D Lead Halide Perovskite by Transient Absorption Spectroscopy
- Version of Record online: 09 December 2024
Review
Advances and Challenges of Single-Pixel Imaging Based on Deep Learning
- Version of Record online: 09 December 2024
An overview of the latest advancements in deep learning technologies in single-pixel imaging is provided. The fundamental principles of single-pixel imaging and deep learning are initially presented. Subsequently, a comprehensive review is conducted on the advancements of deep learning in various domains of single-pixel imaging. Finally, open challenges and potential solutions are discussed.
Research Article
Nanostructured Gold Interlayer-Enhanced Self-Powered Photodetectors for Visible and Long-Wave Infrared Dual-Band Applications
- Version of Record online: 09 December 2024
Inserting nanostructured gold into the interface between the silicon substrate and pyroelectric semiconductor produces several benefits, including light trapping, dark current suppression, enhancement of the intrinsic built-in electric field, and intensification of spontaneous polarization. The resulting p-Si/nanostructured Au/CdS detectors demonstrate high-performance responses to visible and long-wave infrared dual-band without external bias, achieving dual functionality for visible light communication and passive human recognition.
Scalability of Ultralow-Loss Calibration-Free Silicon Photonic Mach-Zehnder Switches
- Version of Record online: 07 December 2024
This Monte Carlo analysis suggests that the considerable random phase imbalance of the switch elements is the dominant fundamental obstacle for scaling up MZS. Therefore, calibration-free MZSs are crucial for scaling up. Also, the scalability of the Benes topology is projected and concludes that it is promising to realize large-scale, low-excess-loss, calibration-free N × N photonic switches (e.g., N ≥ 64) based on the proposed MZS.
Electrically Tunable Spin-Orbit Coupled Photonic Lattice in a Liquid Crystal Microcavity
- Version of Record online: 07 December 2024
A tunable 1D photonic crystal is created with strong polarization dependence by embedding a uniform lying helix in a planar microcavity. Voltage-controlled orientation of liquid crystal molecules alters photonic bandgaps and induces spin-orbit coupling, that can be treated as a non-Abelian gauge potential. Doping with dyes enables tunable dual- and circularly- polarized lasing.
Ultrathin, Wavelength-Multiplexed and Integrated Holograms and Optical Neural Networks Based on 2D Perovskite Nanofilms
- Version of Record online: 06 December 2024
A feasible and promising strategy is developed for achieving highly integrated wavelength-multiplexed diffractive devices. The thickness of the diffractive layer can be decreased to sub-ten nanometers under the condition of pronounced amplitude modulation, and wavelength-multiplexed holograms and optical neural networks with low cross-talks can be realized using selective absorption of 2D perovskites, getting rid of the usage of complex optical structures or filters.
Custom-Shapable and Reusable Thermoplastic Manganese Halide Scintillation Glass for Curved X-Ray Imaging
- Version of Record online: 05 December 2024
A highly transparent and custom-shapable thermoplastic manganese halide scintillation glass is reported by using a facile melt-quenching approach. With the tailored thermoplasticity, the glass is entailed with great adaptability and reusability, which can be molded multiple times to conform to different matters with diverse geometries, achieving consistent high-resolution curved X-ray imaging.
Defects in Ligand-Exchange-Passivated Mixed-Halide Double Perovskite Nanocrystals for X-ray Imaging
- Version of Record online: 05 December 2024
A simple and efficient method is developed, incorporating anion and ligand exchange processes to passivate surface defects and hinder ion migration. This significantly enhances optical and radioluminescence properties of double perovskite nanocrystals. The combination of negligible self-absorption and exceptional X-ray absorption capabilities facilitates an outstanding light yield of ≈20 952 photons MeV−1, a high spatial resolution of 8.1 lp mm−1, and a low detection limit of 207.5 nGyair s−1.
Ultrabroadband Light Coupling for Integrated Photonics via Nonadiabatic Pumping
- Version of Record online: 05 December 2024
A strategy based on nonadiabatic pumping is proposed to realize ultrabroadband light coupling for integrated photonics, which is experimentally demonstrated in thin-film lithium niobate platform. The devices exhibit a 1 dB bandwidth of ≈320 nm, with a coupling length of ≈55 µm. The strategy enables to construct multiple-level cascaded networks for broadband optical interconnections on chip.
Power Clamping in Second Harmonic Generation Within an On-Chip Lithium Niobate Microdisk
- Version of Record online: 05 December 2024
The physical mechanism behind the efficient and powerful power clamping in second harmonic generation is revealed and analyzed. Experimentally, the two distinct power clamping points including the high normalized conversion efficiency of ≈38% mW−1 and the high output power of ≈1.2 mW are separately observed, respectively, consistent with the theoretical model.
Ultrafast Room-Temperature Synthesis of Yb3+/Er3+ Codoped K3ZrF7 Nanocrystals for Thermal Enhancement of Upconversion
- Version of Record online: 04 December 2024
Ultrafast room-temperature synthesis of K3ZrF7:Yb/Er nanocrystals is reported for the first time. These nanocrystals exhibit superior upconversion luminescence to both their high-temperature-synthesized counterparts and the extensively studied NaBiF4:Yb/Er nanocrystals. The K3ZrF7:Yb/Er nanocrystals display thermal enhancement of upconversion over a temperature range from room temperature to 473 K, which can serve as supersensitive nanothermometer for ratiometric temperature sensing.
Correlating Double-Cone Polariton Dynamics with Local Femtosecond Laser Modifications in Ultrashort-Pulse-Stimulated Crystals
- Version of Record online: 04 December 2024
Double-cone emission processes involving of Cherenkov-type phonon polaritons (PhPs) and plasmon-PhPs in ultrashort-pulse-stimulated ferroelectric crystals and graphene are revealed by ultrafast spectroscopy. Transient signals of PhPs can be correlated with femtosecond-laser-induced modifications inside ferroelectric lithium niobates, achieving a PhP threshold criterion for ultrasmooth femtosecond laser nanofabrication. It gives insights into quantum correlations between cone-shape electron wave packets and quantized polaritons.
Quasi-Bound States in the Continuum on Dislocated Bilayer Metal Gratings for Spatiotemporal Vortex Pulse Generation
- Version of Record online: 04 December 2024
This work presents a metasurface method using dislocated two sub-layer gratings to efficiently generate spatiotemporal vortex pulses (STVPs) with transverse orbital angular momentum. This technique exploits quasi-BIC modes, demonstrating experimental validation at microwaves. Furthermore, the method's potential for expansion into the optical range and its capability to generate high-order STVPs through cascading methods are discussed.
High Purcell Factor Driven by Simultaneous Bianisotropy and Anapole State in All-Dielectric Metasurfaces
- Version of Record online: 03 December 2024
The partially slotted dielectric metasurface demonstrates the coexistence of bianisotropy and the anapole state, enhancing both electric and magnetic Purcell factors. This synergy paves the way for novel photonic devices with improved performance, advancing applications in light-matter interactions and optical engineering.
Photostimulated Ultraviolet Luminescence for Anti-Counterfeiting in Daylight Conditions
- Version of Record online: 03 December 2024
Photostimulated luminescence in the ultraviolet (PSL-UV) offers a fresh and effective solution to combating counterfeiting in bright daylight. For instance, NaYF4:Gd3+ phosphor can absorb X-ray energy and subsequently emit UV light when exposed to visible environmental light, demonstrating the exceptional durability and reusability of PSL-UV technology. This approach has the potential to greatly improve security measures across multiple industries.
Highly Efficient Novel Garnet-Structured Yellow Emitting Phosphor for High Power Laser-Driven Lighting
- Version of Record online: 02 December 2024
A novel yellow-emitting phosphor, BaLu2(Mg0.6Al2.8Si1.6)O12:Ce3+, demonstrates a high external quantum efficiency of 66.2%. Integrated into a phosphor wheel, it achieves 3894 lm output with no saturation under high-intensity blue laser excitation, showcasing significant potential for high-power laser-driven lighting applications.
Anapole Plasmonic Meta-Atoms for Nearly Transparent Metamaterials
- Version of Record online: 30 November 2024
The work discusses anapole states in plasmonic nanostructures, which combine the seemingly contradictory properties of strong near-field enhancement with minimal scattering. It explores whether a single planar plasmonic nanostructure can exhibit such properties and serve as a meta-atom for metamaterials. The study presents compact designs that demonstrate this potential, uses multipole decomposition techniques to explain the anapole formation, and demonstrates its applications for nearly transparent metamaterials and tunable nanophotonics.
Review
Two-Dimensional Spiral: A Promising Moiré Superlattice
- Version of Record online: 30 November 2024
A direct synthesis of spiral moiré superlattices (SMSs) from chemical vapor deposition method can be realized, which is attributed to the combination of the screw dislocation-driven growth mechanism and the Euclidean or non-Euclidean substrates. It is possible that completely novel physical properties can be discovered in SMSs and eventually realize industrial applications.
Research Article
Three-Photon Upconversion Luminescence of Gd2O2S: Ho3+, Er3+ for High-Sensitivity FIR Thermometer and Multimode Anti-Counterfeiting
- Version of Record online: 30 November 2024
Based on the three-photon upconversion and energy transfer process, the tunable green-red upconversion luminescence can be realized in Ho3+ and Er3+ co-doped Gd2O2S under the excitation of 1550 nm laser. This multifunctional phosphor can be well applied in various fields such as high-sensitivity (Sr ≈ 2.46% K−1@170 K) fluorescence intensity ratio thermometers, multimode anti-counterfeiting (triple light response), and information encryption.
Efficient Cryogenic Nonlinear Conversion Processes in Periodically-Poled Thin-Film Lithium Niobate Waveguides
- Version of Record online: 30 November 2024
This work provides the first investigation of nonlinear conversion processes in periodically poled thin-film lithium niobate waveguides at cryogenic conditions (7 K). High conversion efficiency at both cryogenic and room temperatures for both classical second-harmonic generation and quantum photon-pair generation processes are experimentally demonstrated. These results facilitate the development of cryogenic nonlinear applications with lithium niobate photonic integrated circuits.
Review
Janus 2D Transition Metal Dichalcogenides: Research Progress, Optical Mechanism and Future Prospects for Optoelectronic Devices
- Version of Record online: 30 November 2024
This review discusses the latest advancements in Janus two-dimensional (2D) transition metal dichalcogenides (TMDCs) including their van der Waals (vdWs) heterostructures, from both theoretical and synthesis perspectives. It summarizes research on their physical characterestics including applications in optoelectronics. Lastly, it presents future directions, and challenges in the Janus 2D TMDCs and their vdWs heterostructures for designing promising optoelectronic devices.
Research Article
Non-Hermitian Loss-driven Broadband Low-Loss on-Chip Terahertz Photonic SPDT Switch
- Version of Record online: 28 November 2024
A non-Hermitian loss-driven all-silicon broadband low-loss on-chip SPDT switch is experimentally demonstrated in the terahertz photonic platform. Both channels of the SPDT switch support on-chip 16-QAM streams with a 36-Gbit s−1 data rate. The designed switch is anticipated as a basic building block for a myriad of on-chip applications, including 6G communications, detection, and sensing.
Tunable Tri-Channel Orthogonal Full-Color Luminescence in Nanostructure toward Anticounterfeiting and Information Security
- Version of Record online: 28 November 2024
This work reports a simple core-shell nanostructure to achieve upconversion/downshifting dual-mode orthogonal red-green-blue (RGB) full-color luminescence. Furthermore, it is able to realize the arbitrarily controllable multicolor output by adopting the multi-wavelengths (980/808/254 nm) selective excitation scheme, exhibiting great application promise in emerging cutting-edge fields such as multiple anticounterfeiting and information security.
High Quality Lithium Niobate Euler Racetrack Resonators
- Version of Record online: 28 November 2024
Euler racetrack micro-cavity based on X-cut and Z-cut thin-film lithium niobate (TFLN) is demonstrated in simulation and experiment. The Euler microcavity shows great performance in quality factor improving and mode-crossing suppressing. The method paves the way for electro-optical (EO) comb generation and high-performance integrated device fabrication.
Reconfigurable Generation and Spin Manipulation of Structured Beams Based on Cascaded Liquid Crystal Pancharatnam–Berry Phase Elements
- Version of Record online: 28 November 2024
Reconfigurable generation of various forms of typical structured beams is realized using two cascaded liquid crystal Pancharatnam–Berry phase elements. Different output modes are switched via rotating and/or translating the elements, instead of using complex, delicate modulation devices. Such mechanically operative optical elements not only avoid expenditure on computer-controlled devices, but also bring flexibility in spin-photonic manipulation.
A Reconfigurable Metasurface Antenna for Arbitrarily Polarized Beam Generation and Advanced Polarization Detection
- Version of Record online: 28 November 2024
A reconfigurable metasurface antenna (RMA) that can be used as a full polarized beam launcher to generate arbitrarily polarized radiation waves, or as a polarization detector to identify the arbitrary polarization states of unknown incoming waves is proposed. It has the advantages of high accuracy and quick response, which is promising to apply in future intelligent sensing systems.
Broadband Rapid Polarization Manipulation and Imaging Based on Pancharatnam-Berry Optical Elements
- Version of Record online: 28 November 2024
This paper proposed a rapid polarization manipulation method based on PBOEs and integrated the module into imaging systems. The frequency of polarization manipulation can reach 899 Hz. With the minimum change of traditional imaging systems, polarization imaging is achieved with both high spatial resolution and imaging speed. it shows great potential in both microscopic and telescopic imaging.
Coherent Control of Relativistic Electron Dynamics in Plasma Nanophotonics
- Version of Record online: 27 November 2024
A novel approach to controlling relativistic electron dynamics in intense femtosecond laser-plasma interactions is proposed by tailoring solid-dense plasma at the nanoscale. Plasma nanoengineering enables the space-time manipulation of local laser fields that drive electron dynamics. This control is demonstrated to generate attosecond electron bunches, enhance in-phase electron acceleration, and enable directional steering of the electron beam over a wide angular range.
Super-Large Field-of-View, High-Accurate and Real-Time 3D Scene Reconstruction Based on Metasurface-Enabled Structured Light
- Version of Record online: 27 November 2024
This research is motivated by how to build a practical 3D scene reconstruction application based on metasurfaces. Specifically, a metasurface enabled structural-light platform is established, with which one can realize both wide-field, high-accuracy and video-rate 3D reconstruction, while remains an ultracompact volume.
Silicon-Nitride-Integrated Hybrid Optical Fibers: A New Platform for Functional Photonics
- Version of Record online: 27 November 2024
A novel silicon-nitride-integrated hybrid fiber platform is demonstrated. Ultra-uniform silicon-nitride nanolayer is coated around the entire microfiber circumference with a sub-nm roughness. Precisely tunable silicon-nitride nanolayer thickness enables mode hybridization between nanolayer and fiber core modes, resulting in rich dispersion landscapes. A flat supercontinuum spectrum spanning >1.5 octaves (−20 dB level) is generated through optimizing the nanolayer thickness.
Asymmetric Domain Growth for Bistable Information Hiding and Revealing in Blue Phase Liquid Crystals
- Version of Record online: 26 November 2024
Bistable information hiding and revealing is realized through asymmetric domain growing of a blue phase liquid crystal. By leveraging photopatterned alignment techniques and temperature gradients, reversible information hiding and revealing of both near-field quick response (QR) code patterns and far-field diffraction is demonstrated. It provides a promising strategy for optical security.
Magnetoplasmonic Gratings Induced an Unusual Magneto-Optical Kerr Effect at Optical Frequencies
- Version of Record online: 25 November 2024
The Fe-based grating nanostructure proposed in this work displays the highest peak value of s-polarized TMOKE at optical frequencies to date, resulting from the excitation of surface plasmon polaritons (SPPs). The intensity of s-polarized TMOKE can be further increased by the deposition of Al2O3, and it exhibits highly sensitive sensing performance to the changes in the surrounding environment.
Observation and Manipulation of Self-Chaos in Disordered Optical System
- Version of Record online: 25 November 2024
The dynamical evolution process of self-chaos in disordered optical system is observed, and self-chaotic behavior can be flexibly manipulated by altering the interaction strength among random modes. Simultaneously, by adopting Erbium-Raman hybrid gain, chaotic bandwidth is synergistically enhanced to 38 GHz, which is successfully employed for higher-speed true random bits generation and a scheme of local information encryption with higher-quality.
High-Gain, High-Order Vortex Air Lasing Generated by Plasma Amplification
- Version of Record online: 25 November 2024
Vortex air lasing with a tunable vortex order from the first to the tenth order is produced through vortex seed amplification in plasma. The amplified signal shows the same topological charge as the seed, a doughnut-shaped profile, and the amplification factor up to 104. Such vortex beams hold great potential in standoff detection of chiral molecules and rotating objects.
A Space-Time Knife-Edge in Epsilon-Near-Zero Films for Ultrafast Pulse Characterization
- Version of Record online: 23 November 2024
A space-time knife edge utilizes the temporal-resolution of femtosecond autocorrelation and the spatial-resolution of beam deflection to creatively characterize parameters of an ultrashort laser pulse. Practically, this leverages epsilon-near-zero materials for their strong refractive index nonlinearity facilitating easy calibration and calculation.
Thin-Film-Lithium-Niobate Photonic Chip for Ultra-Wideband and High-Precision Microwave Frequency Measurement
- Version of Record online: 23 November 2024
An ultra-wideband, high-precision integrated photonic instantaneous frequency measurement (IFM) system on a thin-film lithium niobate (TFLN) platform is demonstrated. The system integrates a high-speed intensity modulator, a high-Q microring resonator, and dual-stage asymmetrical MZIs for coarse wide-band and precise narrow-band measurements. It can identify various microwave signals across a wide frequency range up to 67 GHz with an RMS error below 123 MHz, advancing broadband microwave photonics.
Ultrahigh-Power Germanium Photodetector Enabling Amplifier-Free Wireless Communication
- Version of Record online: 22 November 2024
The photodetectors (PD) are indispensable components in microwave photonics. This work presents an ultrahigh-power germanium PD with an unprecedented photocurrent of 471.4 mA, being achieved through enhanced optical absorption and improved photogenerated carrier transit. The high-power performance enables an amplifier-free wireless communication, and represents a significant advancement toward high-quality fiber-wireless access network.
Reconfiguration of Quantum Photonic Integrated Circuits Using Auxiliary Fields
- Version of Record online: 22 November 2024
This research presents a novel approach for reconfiguring quantum photonic integrated circuits using auxiliary fields introduced via femtosecond laser direct writing. The method allows precise control of phase shifts and waveguide coupling, demonstrated by high-fidelity quantum logic operations (CNOT and C-PHASE gate conversions) and error correction. This technique promises advancements in large-scale integrated quantum circuits and complex photonic quantum networks.
Low-Loss and Low-Power Silicon Ring Based WDM 32100 GHz Filter Enabled by a Novel Bend Design
- Version of Record online: 22 November 2024
Switchable Narrowband Diffuse Thermal Emission With an In3SbTe2-Based Planar Structure
- Version of Record online: 22 November 2024
The study presents a planar reconfigurable thermal emitter based on phase-change material In3SbTe2, achieving high narrowband emissivity in the amorphous phase and low broadband emissivity in the crystalline phase. The design results in angle- and polarization-independent emission, allowing for centimeter-scale programmable patterns with a resolution of 20 µm, with applications in labeling and anticounterfeiting.
Highly Reversible Tuning of Light-Matter Interactions in Van der Waals Materials Coupled with Hydrogel-Assisted Optical Cavity
- Version of Record online: 19 November 2024
This study focuses on controlling light-matter interactions using cavity systems with adjustable coupling based on dielectric-hydrogel-metal resonators without requiring nanopositioning or lithography. By manipulating the tungsten disulfide layer thickness, the flexible manipulation of weak-intermediate-strong transitions was demonstrated. The coupling strength can be reversibly tailored by modulating the resonator's dry/immersed states, offering potential applications in polariton lasing, switches, and sensors.
Highly Intelligent Forward Design of Metamaterials Empowered by Circuit-Physics-Driven Deep Learning
- Version of Record online: 19 November 2024
This work introduces a circuit-theory-informed neural network (CTINN) that significantly enhances the generalization capability in spectral prediction and metamaterial design. The CTINN incorporates physical insights of equivalent circuits into the deep learning model, leading to superior accuracy with fewer training samples versus the conventional data-driven method. This scheme shows great potential to develop smarter deep-learning applications in metamaterial development.
Regulating Second-Harmonic Generation in 2D Chiral Perovskites Through Achiral Organic Spacer Cation Alloying Strategy
- Version of Record online: 16 November 2024
Using an achiral organic spacer cation alloying strategy, a series of 2D chiral perovskites are constructed. This strategy can not only effectively regulate the second-harmonic generation (SHG) of the 2D chiral perovskites, but also provide convenience to reveal the relationship between SHG and self-trapped exciton emission. In addition, their microscopic images of circularly polarized SHG are provided.
A Polarization-Insensitive and Adaptively-Blazed Meta-Grating Based on Dispersive Metasurfaces
- Version of Record online: 16 November 2024
Meta-gratings inspired by orthogonal harmonic oscillations (OHO) enable precise control of phase dispersion, allowing broadband, polarization-insensitive diffraction. The adaptive blaze angles enhance diffraction efficiency across wavelengths from 8.7 to 12.2 µm, achieving ≈80% efficiency and less than 4.6% polarization-dependent variation. This approach holds promise for applications in spectrometry, broadband beam steering, and hyperspectral imaging.
Efficient Simultaneous Second Harmonic Generation and Dispersive Wave Generation in Lithium Niobate Thin Film
- Version of Record online: 16 November 2024
The efficient simultaneous generation of second-harmonic and dispersive waves is demonstrated in lithium niobate thin films by leveraging both the effects of second and third-order nonlinearities under near-visible wavelength pumping. This approach offers a simple and viable pathway for achieving high-energy, flat UV–vis—NIR supercontinuum generation on-chip.
Pyroelectrically Driven Charge Transfer and its Advantages on SERS and Self-Cleaning Property
- Version of Record online: 16 November 2024
This research prepared Ag/Graphene/BaTiO3 composite SERS substrates, which successfully utilized the pyroelectric field excited by the materials to achieve an ultrasensitive SERS signal response, effectively solving the self-cleaning problem. Meanwhile, the charge transfer pathway is analyzed rigorously. It confirms that enhancing the charge transfer process is an effective way to enhance the SERS response.
Plasmon–Exciton–Polariton Condensation in Organic Semiconductor-Covered Plasmonic Lattices
- Version of Record online: 16 November 2024
Condensation of plasmon–exciton–polaritons (PEPs)in the blue wavelength region is achieved through integrating a neat film of organic semiconductors onto plasmonic lattices to mitigate metal losses. By tailoring the band structures of plasmonic lattices, the condensation of PEPs is successfully manipulated into different energy states, offering valuable insights for advancing PEP systems and of all-optical polaritonic devices.
Large Optical Nonlinearity Enhancement and All-Optical Logic Gate Implementation in Silver-Modified Violet Phosphorus
- Version of Record online: 16 November 2024
The enhanced spatial self-phase modulation (SSPM) effect in silver-modified violet phosphorus (Ag-VP). The SSPM enhanced mechanism in Ag-VP is that Ag-modified VP exhibits some flat impurity levels (i.e. impurity state) within the forbidden band, leading to higher electron excitation efficiency and improved light–matter interaction, ultimately enhancing the SSPM response.
Dark Current Suppression in Two-dimensional Histamine Lead Iodine Perovskite Single Crystal for X-ray Detection and Imaging
- Version of Record online: 16 November 2024
In this study, a vertical structure detector is fabricated by using a 2D histamine lead halide perovskite single crystal. The device achieves high-sensitivity X-ray detection and imaging, primarily due to effective dark current suppression, which is enabled by the short interlayer distances, the dielectric screening effect of diamine, and the optimized high crystal quality of the histamine lead iodine crystals.
Optothermal-Enabled Reconfigurable Colloidal Photonic Crystals for Color and Spectrum Manipulation
- Version of Record online: 16 November 2024
This study addresses the challenge of spatial reconfigurability in colloidal photonic crystals (CPCs) by introducing an optically induced thermoelectric field. It enables the efficient formation of CPCs with high reconfigurability, advancing their potential for broader applications in reconfigurable photonics chips and colloidal science.
Angle-Based Neuromorphic Wave Normal Sensing
- Version of Record online: 15 November 2024
The Shack–Hartmann Wavefront Sensor dynamic range (DR) taxonomy is extended by introducing a Type III DR from the perspective of wave normal. NeuroSH, an event-based framework, surpasses the curvature constraint in angle-based model by approximating the wave normal as 3D spot trajectories within the spatiotemporal neighborhood. With its asynchronous nature, NeuroSH demonstrates superiority in long-term diagnosing ultra-fast, large-gradient, turbulence.
Topological Metasurface for Spin-Decoupled Wavefront Manipulation of Terahertz Surface Plasmons
- Version of Record online: 15 November 2024
A topological metasurface for near-field control has been developed based on the exceptional topological phase derived from the parameter space of chiral double-split ring resonators. By integrating a leaky mode design, the metasurface's capability for spin-decoupled wavefront manipulation of terahertz surface plasmons is demonstrated experimentally.
Review
Volumetric Imaging From Raman Perspective: Review and Prospect
- Version of Record online: 15 November 2024
This review explores recent achievements in 3D visualization of biological samples from the Raman perspective, including scanning mechanisms, light sheets, tomography strategy, compressive sensing, holography, and tissue clearing. These technologies enable the imaging of chemical constituents and the distribution of samples in a whole volume, potentially offering a strategy to accelerate new discoveries across diverse fields of research.
Research Article
Precise Genotyping Via Surface-Enhanced Raman Spectroscopy-Based Optical Sensing Chip for Guiding Targeted Therapy in Lung Cancer
- Version of Record online: 15 November 2024
A bio-sensing platform based on surface-enhanced Raman scattering is designed for genotyping of lung cancer-related circulating tumor DNA, enabling precise screening of populations benefiting from targeted therapy and guiding therapeutic decisions. Moreover, this liquid biopsy technology can be integrated with portable Raman scanning system to develop a compact genotyping instrument that it is of imperative clinical value for personalized medicine.
Efficient and Stable Quantum-Dot Light-Emitting Diodes with Trilayer PIN Architecture
- Version of Record online: 15 November 2024
Efficient quantum-dot light-emitting diodes (QLEDs) with a novel trilayer PIN architecture are developed using Spiro-OMeTAD:TFB bulk-heterojunction (BHJ) hole transport layer (HTL). Due to the enhanced hole injection and suppressed electron leakage of the Spiro-OMeTAD:TFB BHJ HTL, the resulting trilayer PIN QLEDs can exhibit excellent external quantum efficiency of 25.1% with an Al electrode and 27.3% with an EGaIn electrode.
CsPbX3@Glass (X = Cl, Br, I) Nanocomposites with Whole-Family High Absorption Efficiency above 75% for Backlit Display
- Version of Record online: 15 November 2024
CaO additive is evidenced to break the bridging oxygen bond of [SiO4] and depolymerize glass network. This will promote in situ precipitation of green and red CsPbX3 (X3 = Br3, Br1I2) PeQDs in borosilicate glass with record absorption efficiency and external quantum efficiency of 81% & 75% and 78% & 67%, paving the way for realizing commercial application of ultra-stable CsPbX3@glass-converted backlit display.
Wide-Temperature Persistent Luminescence
- Version of Record online: 15 November 2024
The X-ray-induced Frenkel defects are dynamically present and recoverable. By leveraging these defects and doping various rare-earth ions into NaLuF4 phosphors, the multicolored persistent luminescence (PersL) has been achieved across an extensive temperature range from 77 to 500K. This discovery enhances the understanding of X-ray-induced PersL, potentially setting the groundwork for future applications in extreme conditions.
Regulating A-Site Alloying of Te4+-Doped Hafnium-Halide Perovskite for Fluorescence Thermometry Achieving Breakthrough Sensitivity at High Temperatures
- Version of Record online: 15 November 2024
A series of Rb2−xCsxHfCl6: y% Te4+ is synthesized via A-site regulation. The Rb2HfCl6:2% Te4+ sample, with the lowest activation energy, exhibits rapid lifetime decay at high temperatures, achieving a breakthrough thermal sensitivity of 20.69% K−1 at 390 K. Moreover, a noncontact high-temperature warning system is designed for lubricating oil pipelines, enhancing the safety and efficiency of ship power systems.
Generalized Coherent Wave Control at Dynamic Interfaces
- Version of Record online: 15 November 2024
Coherent wave control oftentimes requires identical frequencies or wavevectors of associated incidences. A generalized coherent wave control is proposed at the spatiotemporally engineered medium with a dynamic interface. The proposed platform allows the interference between scattered waves regardless of their different frequencies and wavevectors. The findings thus hold promise for sculpting light with light with enhanced freedoms.
Multi-Color Optical Quasiparticle Laser Source Formed of a Pr3+ Doped Fiber Laser with a Dual-Output Coupling Geometry
- Version of Record online: 12 November 2024
Multicolor visible optical quasiparticles (bimerons and skyrmions) source is demonstrated by employing a diode-pumped Pr3+-doped fluoro-aluminate glass (Pr3+: WPFG) fiber laser with a wedge-output coupler. This robust and cost-saving system explores potentially innovative applications in materials science and biotechnologies.
Direct Linearly Polarized Emission in van der Waals LEDs via Flexoelectric Effect
- Version of Record online: 12 November 2024
A direct emission of linearly polarized light from van der Waals light–emitting diodes (vdWLEDs) can be observed at room temperature in the visible range, which is attributed to the flexoelectric effects induced by the manually designed non-uniform strain in monolayer transition metal dichalcogenides.
Near-Infrared Dual-Band Frequency Comb Generation from a Silicon Resonator
- Version of Record online: 11 November 2024
Near-infrared dual-band frequency combs are demonstrated at the pump and Stokes wavelengths using a silicon multimode resonator, which is realized through stimulated Raman scattering and nondegenerate four-wave mixing between the pump and Stokes fields. The work can find potential applications in optical telecommunications, sensing, and quantum metrology in the telecom band using a monolithic single silicon chip.
Highly Efficient Flexible Antimony Halide Scintillator Films with In Situ Preparation for High-Resolution X-Ray Imaging
- Version of Record online: 11 November 2024
An in situ fabrication strategy is proposed to prepare flexible scintillator film based on organic–inorganic hybrid antimony halide C38H36P2SbCl5 (MTP2SbCl5) with low light scattering performance. The low light scattering greatly inhibits optical crosstalk in X-ray imaging, effectively improving the spatial resolution of MTP2SbCl5 film from 4.5 to 10.2 lp mm−1. On this basis, high-quality X-ray imaging for irregular objects are achieved.
Hyper-Sampling Imaging by Measurement of Intra-Pixel Quantum Efficiency Using Steady Wave Field
- Version of Record online: 11 November 2024
A novel method for measuring intra-pixel quantum efficiency using a steady wave field is introduced, enabling the reconstruction of high-quality super-resolution images. This technique has the potential to enhance the sampling limit of conventional digital image sensors by a factor of 4 × 4 times, or even more, surpassing the original pixel resolution.
Review
Advancing the Commercialization of Perovskite-Based Radiation Detectors for High-Resolution Imaging
- Version of Record online: 11 November 2024
Perovskite has shown excellent performance in the field of high-energy radiation detection. However, many challenges remain to be overcome before realizing the commercialization, including the optimization for properties of perovskite material, the improvement for the interface of electrode/perovskite, and the design for array detectors. This review focuses on these issues and provides feasible routes for achieving high-performance perovskite-based radiation detectors.
Research Article
Suppressing the Dark Current Under Forward Bias for Dual-Mode Organic Photodiodes
- Version of Record online: 11 November 2024
The principle of energy level alignment followed by traditional organic photodiodes is weakened by adopting an interface layer of PEIE-Co with deep energy level and abundant carrier traps. The device dark current is efficiently suppressed under forward bias, and a bias-switchable organic photodiode that integrates photoconductive and photomultiplication modes is realized, demonstrating potential in adaptive detection of weak and strong light.
Polarization Volume Hologram for On-Chip Wavefront Engineering
- Version of Record online: 11 November 2024
In this work, the liquid crystal on-chip wavefront control strategy is proposed and experimentally demonstrated. This strategy can realize wavefront engineering of converting guidedwaves into free-space light by ingeniously designing the initial phase of the polarization volume grating. The liquid crystal on-chip wavefront engineering may find applications in freeform optics, near-eye displays, LIDAR, and integrated photonic systems.
Ultra-Broadband Visible-DUV Supercontinuum Generation by Non-Resonant Coherent Raman Scattering in Air
- Version of Record online: 09 November 2024
This paper presents a novel approach of non-resonant coherent Raman scattering (CRS) to generate ultra-broadband visible-DUV supercontinuum in ambient air, in which the non-resonant CRS serves as spectral bridges to link the neighboring Raman pump laser spectra in air media with rovibrational coherence of molecules created by the coherence pump laser.
Regulating Broadband Near-Infrared Mechanoluminescence via Energy-Level Engineering for Potential Biomechanical Imaging
- Version of Record online: 09 November 2024
The chemical co-substitution method [Ca2++Ge4+] → [Y3++Ga3+] strategy is used to regulate the local crystal field to realize Cr3+/Nd3+ co-doped ultra-wideband near infrared spectral I (650-1000 nm) mechanoluminescence. Combined with first-principles calculations, the effects of different defect types on the electronic structure are researched in detail, and the biostress sensing potential applications is demonstrated.
Grating-Based Eight-Channel Lan-WDM Silicon Photonic Transceiver for Tb/s Applications
- Version of Record online: 07 November 2024
A grating-based eight-channel local-area-network wavelength division multiplexing silicon photonic transceiver is designed and demonstrated for Tb/s applications. With a fiber array packaged, a B2B data capacity of 1.56 and 1.42 Tb/s is demonstrated for the transmitter and receiver, respectively. In transceiver mode, the B2B data capacity is decreased to 1.18 Tb/s. Two and 10 km SMF transmission experiments are also carried out.
In-Plane Metasurface Design for Perfect Chiral Dichroism in Inhomogeneous Environment
- Version of Record online: 07 November 2024
This work introduces a chiral metasurface capable of perfectly converting one circular polarization into another in a non-uniform environment. The perfect unitary circular conversion reflectance is achieved through the coupling of two dipole bound states in the continuum, supported by a periodic structure whose unit cell consists of four dielectric nanoparticles.
High-Resolution X-Ray Imaging With 0D Organic–Metal Halide Scintillator Featuring Reversed Exciton Trapping
- Version of Record online: 07 November 2024
The scale-up inorganic–organic hybrid halide manganese scintillation nanocrystals are prepared through simple rotary evaporation method. These nanocrystals exhibit intrinsic thermally excited exciton emissions, displaying thermal expansion before overcoming trap levels and negative thermal expansion afterward. The flexible scintillation film that is prepared with nanocrystals and PDMS can be applied to high-resolution X-ray imaging.
Multi-Wavelength Achromatic Graphene Metalenses for Visible, NIR, and Beyond
- Version of Record online: 07 November 2024
Based on a partial intensity resonance mechanism, requiring no iterative algorithms, multi-wavelength achromatic metalenses covering ultrabroad wavebands, including the visible and near-infrared are proposed and demonstrated. Two achromatic graphene metalenses, with less than 0.15% of the desired focal length values for visible and communication bands, are designed and fabricated. Clear and high-quality images of microscopic character and Brassica napus cells are obtained.
Ethanol-Induced Reversible Phase Transition in Antimony Halides for Morse Code Anti-Counterfeiting and Optical Logic Gates
- Version of Record online: 07 November 2024
Two antimony-based halides, (C21H21P)2SbCl5 and (C22H24P)2SbCl5, are synthesized using different organic cations. Both compounds exhibit bright orange–yellow emissions with a PLQY of 82.6% and 83.5%, respectively. While (C21H21P)2SbCl5 maintains stable orange–yellow luminescence when exposed to ethanol, (C22H24P)2SbCl5 undergoes a structural transformation to non-luminescent (C22H24P)2Sb2Cl8 upon ethanol treatment, which could be reverted to its luminescent state by heating.
Steering Nonlinear Chiral Valley Photons Through Optical Orbit–Orbit Coupling
- Version of Record online: 06 November 2024
The research demonstrates the directional coupling of nonlinear chiral valley photons in monolayer tungsten disulfide using optical orbit–orbit coupling at room temperature. The coupling direction is controlled by the helicity of the fundamental-frequency pumping light. The findings not only provide a novel method for manipulating the valley's degree of freedom but also enhance the flexibility of directing valley emission.
Detection of Nonlinearity in Photonic Lattices
- Version of Record online: 06 November 2024
An approach is proposed to detect the nonlinearity of photonic lattices in a direct way. By properly launching Airy beams into the lattices, one can directly obtain the nonlinear response function of the discrete system in the nonlinearly-shaped beam profiles. This method is expected to trigger more ideas for measuring the nonlinearity of optical periodic structures via other structured lights.
Large-Area Floating Display with Wafer-Scale Manufactured Metalens Arrays
- Version of Record online: 05 November 2024
Exciton Dissociation and Long-Lived Delayed Components in High-Efficiency Quasi-Two-Dimensional Green Perovskite Light-Emitting Diodes
- Version of Record online: 05 November 2024
An intrinsic characteristic of perovskites with a long-lived delayed component spanning hundreds of microseconds associated with exciton dissociation is first observed in perovskite emitters. Benefiting from the incorporation of 18-crown-6 and tris(4-fluorophenyl)phosphine oxide, trap-assisted nonradiative recombination and exciton dissociation are suppressed, resulting in high-efficiency quasi-two-dimensional green PeLEDs with maximum EQE of 28.9%.
Photoactivated Multicolor Organic Phosphorescence in Intrinsically Stretchable, Self-Healable and Recyclable Polymers
- Version of Record online: 05 November 2024
This work presents the straightforward one-pot photo-initiated copolymerization strategy to fabricate photoactivated persistent RTP polymers with multicolored afterglow, excellent stretchability, and self-healing properties. Utilizing these photoactivated and stretchable persistent RTP polymers, dual encryption can be achieved under UV irradiation and stretching conditions, thereby enhancing the security levels of the stored confidential information.
Review
Noise-Like Pulse Seeded Supercontinuum Generation: An In-Depth Review For High-Energy Flat Broadband Sources
- Version of Record online: 04 November 2024
NLP 4 Continuum: This review highlights the unique capabilities of noise-like pulses (NLPs) from passively mode-locked fiber lasers and their potential role in enhanced supercontinuum generation (SCG). It explores NLP characteristics, compares experimental results, and discusses their benefits over conventional ultrashort pulse schemes owing to their relatively higher energies and wider spectrum. NLP-seeded SCG can significantly advance technologies across the biomedical and industrial domains with broader, flatter continua.
Research Article
Fast Gain Dynamics in Interband Cascade Lasers
- Version of Record online: 04 November 2024
Interband Cascade Lasers (ICL) are a versatile technological platform in the mid-infrared spectral domain. Ongoing research pursues the emission of ultrashort pulses via passive mode-locking. Pump-probe measurements on the ICL gain demonstrate that 60–70% of its dynamic behavior is characterized by a rapid recovery time of 2 ps. These findings explain why passive mode-locking has not succeeded so far and strategies toward ICL pulses are proposed.